Behavior of Helium Release from Simulated Radioactive Waste Glasses

Seichi Sato; Hirotaka Furuya; Koshi Morikawa; Masayasu Sugisaki; Yaohiro Inagaki

doi:10.3327/jnst.27.343

Behavior of Helium Release from Simulated Radioactive Waste Glasses

Seichi Sato, Hirotaka Furuya, Koshi Morikawa, Masayasu Sugisaki, Yaohiro Inagaki

Quantum Sciences of Materials

Research output: Contribution to journal › Article › peer-review

Abstract

Rates of He release from two kinds of simulated high-level radioactive waste glasses were measured in the temperature range from 573 to 753 K by a mass spectrometric method. Diffusion coefficients of He in the glasses were determined from the fractional release data. The diffusion coefficients were given as a function of temperature by the equations: In addition, solubilities of He in the glasses were determined from the measurement of the total amount of released He and found to be at 693 K and 1.7xl0⁵ Pa He. The diffusivities and solubilities of He in the glasses were, respectively, several and an order of magnitude lower than silica, alkali silicate and Pyrex glasses, which properties are notable for the radioactive waste glasses.

Original language	English
Pages (from-to)	343-349
Number of pages	7
Journal	journal of nuclear science and technology
Volume	27
Issue number	4
DOIs	https://doi.org/10.3327/jnst.27.343
Publication status	Published - Jan 1 1990

All Science Journal Classification (ASJC) codes

Nuclear and High Energy Physics
Nuclear Energy and Engineering

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title = "Behavior of Helium Release from Simulated Radioactive Waste Glasses",

abstract = "Rates of He release from two kinds of simulated high-level radioactive waste glasses were measured in the temperature range from 573 to 753 K by a mass spectrometric method. Diffusion coefficients of He in the glasses were determined from the fractional release data. The diffusion coefficients were given as a function of temperature by the equations: In addition, solubilities of He in the glasses were determined from the measurement of the total amount of released He and found to be at 693 K and 1.7xl05 Pa He. The diffusivities and solubilities of He in the glasses were, respectively, several and an order of magnitude lower than silica, alkali silicate and Pyrex glasses, which properties are notable for the radioactive waste glasses.",

author = "Seichi Sato and Hirotaka Furuya and Koshi Morikawa and Masayasu Sugisaki and Yaohiro Inagaki",

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AU - Sato, Seichi

AU - Furuya, Hirotaka

AU - Morikawa, Koshi

AU - Sugisaki, Masayasu

AU - Inagaki, Yaohiro

PY - 1990/1/1

Y1 - 1990/1/1

N2 - Rates of He release from two kinds of simulated high-level radioactive waste glasses were measured in the temperature range from 573 to 753 K by a mass spectrometric method. Diffusion coefficients of He in the glasses were determined from the fractional release data. The diffusion coefficients were given as a function of temperature by the equations: In addition, solubilities of He in the glasses were determined from the measurement of the total amount of released He and found to be at 693 K and 1.7xl05 Pa He. The diffusivities and solubilities of He in the glasses were, respectively, several and an order of magnitude lower than silica, alkali silicate and Pyrex glasses, which properties are notable for the radioactive waste glasses.

AB - Rates of He release from two kinds of simulated high-level radioactive waste glasses were measured in the temperature range from 573 to 753 K by a mass spectrometric method. Diffusion coefficients of He in the glasses were determined from the fractional release data. The diffusion coefficients were given as a function of temperature by the equations: In addition, solubilities of He in the glasses were determined from the measurement of the total amount of released He and found to be at 693 K and 1.7xl05 Pa He. The diffusivities and solubilities of He in the glasses were, respectively, several and an order of magnitude lower than silica, alkali silicate and Pyrex glasses, which properties are notable for the radioactive waste glasses.

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Behavior of Helium Release from Simulated Radioactive Waste Glasses

Abstract

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