Magnetic Weyl semimetals are quantum phases of matter arising from the interplay of linearly dispersive bands, spin-orbit coupling, and time reversal symmetry breaking. This can be realised, for example, in Co3Sn2S2, based on a cobalt kagome lattice and characterised by intriguing phenomena such as large anomalous Hall effect, Nernst effect, and water oxidation. Here, we attempt to determine the robustness of the twofold necessary conditions for the emergence of the magnetic Weyl semimetal phase in Co3Sn2S2 ultrathin films. Except for two-dimensional layered materials, a reduction of thickness generally makes it difficult to develop topological character and ferromagnetic long-range order. In Co3Sn2S2 films, while ferromagnetic ordering appears robustly even in average thicknesses of one or two unit cells with island-like polycrystalline domains, the anomalous Hall conductivity appears only above a critical thickness of approximately 10 nm. The emergence of surface conduction and large anomalous Hall effect implies the distinct contribution of Weyl nodes and their Berry curvature. These findings reveal an exotic feature of Weyl physics in thin-film based superstructures as well as a potential for future applications in electronic devices.
All Science Journal Classification (ASJC) codes
- Materials Science(all)
- Mechanics of Materials