Deuterium/tritium behavior in Flibe and Flibe-facing materials

R. A. Anderl, S. Fukada, G. R. Smolik, R. J. Pawelko, S. T. Schuetz, J. P. Sharpe, B. J. Merrill, D. A. Petti, H. Nishimura, T. Terai, S. Tanaka

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Abstract

Experimental studies to investigate the behavior of deuterium and tritium in the molten salt Flibe (2LiF·BeF2), have been conducted as part of the Japan-US joint research program (JUPITER-II). Measurements of deuterium transport were made in a cylindrically symmetric, dual permeation probe assembly containing 400 cc of Flibe. An exact analytical transport solution in cylindrical coordinates was fit to the measured permeation data, and this analysis derived deuterium diffusion and solubility coefficients of 8.0×10-10 m2/s and 3.1×10-4 mol/m3Pa at 600 °C, respectively, and 3.0×10-9 m2/s and 1.0×10-4 mol/m3Pa at 650 °C. The diffusion coefficients were about a factor of two less than previous results derived from capillary-reservoir diffusion measurements with tritium. Solubility results were significantly greater than previously measured for D2 but they were comparable to those for DF in Flibe. The results suggest that the dominant deuterium transport species in Flibe was D +F- for these experiments.

Original languageEnglish
Pages (from-to)1327-1331
Number of pages5
JournalJournal of Nuclear Materials
Volume329-333
Issue number1-3 PART B
DOIs
Publication statusPublished - Aug 1 2004
EventProceedings of the 11th Conference on Fusion Research - Kyoto, Japan
Duration: Dec 7 2003Dec 12 2003

All Science Journal Classification (ASJC) codes

  • Nuclear and High Energy Physics
  • Materials Science(all)
  • Nuclear Energy and Engineering

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    Anderl, R. A., Fukada, S., Smolik, G. R., Pawelko, R. J., Schuetz, S. T., Sharpe, J. P., Merrill, B. J., Petti, D. A., Nishimura, H., Terai, T., & Tanaka, S. (2004). Deuterium/tritium behavior in Flibe and Flibe-facing materials. Journal of Nuclear Materials, 329-333(1-3 PART B), 1327-1331. https://doi.org/10.1016/j.jnucmat.2004.04.220