Effectiveness of paper-structured catalyst for the operation of biodiesel-fueled solid oxide fuel cell

Tran Quang-Tuyen; Taku Kaida; Mio Sakamoto; Kazunari Sasaki; Yusuke Shiratori

doi:10.1016/j.jpowsour.2015.02.116

Effectiveness of paper-structured catalyst for the operation of biodiesel-fueled solid oxide fuel cell

Tran Quang-Tuyen, Taku Kaida, Mio Sakamoto, Kazunari Sasaki, Yusuke Shiratori

Hydrogen Utilization Engineering

Research output: Contribution to journal › Article › peer-review

10 Citations (Scopus)

Abstract

Mg/Al-hydrotalcite (HDT)-dispersed paper-structured catalyst (PSC) was prepared by a simple paper-making process. The PSC exhibited excellent catalytic activity for the steam reforming of model biodiesel fuel (BDF), pure oleic acid methyl ester (oleic-FAME, C₁₉H₃₆O₂) which is a mono-unsaturated component of practical BDFs. The PSC exhibited fuel conversion comparable to a pelletized catalyst material, here, conventional Ni-zirconia cermet anode for solid oxide fuel cell (SOFC) with less than one-hundredth Ni weight. Performance of electrolyte-supported cell connected with the PSC was evaluated in the feed of oleic-FAME, and stable operation was achieved. After 60 h test, coking was not observed in both SOFC anode and PSC.

Original language	English
Article number	20745
Pages (from-to)	320-327
Number of pages	8
Journal	Journal of Power Sources
Volume	283
DOIs	https://doi.org/10.1016/j.jpowsour.2015.02.116
Publication status	Published - Jun 1 2015

All Science Journal Classification (ASJC) codes

Renewable Energy, Sustainability and the Environment
Energy Engineering and Power Technology
Physical and Theoretical Chemistry
Electrical and Electronic Engineering

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title = "Effectiveness of paper-structured catalyst for the operation of biodiesel-fueled solid oxide fuel cell",

abstract = "Mg/Al-hydrotalcite (HDT)-dispersed paper-structured catalyst (PSC) was prepared by a simple paper-making process. The PSC exhibited excellent catalytic activity for the steam reforming of model biodiesel fuel (BDF), pure oleic acid methyl ester (oleic-FAME, C19H36O2) which is a mono-unsaturated component of practical BDFs. The PSC exhibited fuel conversion comparable to a pelletized catalyst material, here, conventional Ni-zirconia cermet anode for solid oxide fuel cell (SOFC) with less than one-hundredth Ni weight. Performance of electrolyte-supported cell connected with the PSC was evaluated in the feed of oleic-FAME, and stable operation was achieved. After 60 h test, coking was not observed in both SOFC anode and PSC.",

author = "Tran Quang-Tuyen and Taku Kaida and Mio Sakamoto and Kazunari Sasaki and Yusuke Shiratori",

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AU - Quang-Tuyen, Tran

AU - Kaida, Taku

AU - Sakamoto, Mio

AU - Sasaki, Kazunari

AU - Shiratori, Yusuke

PY - 2015/6/1

Y1 - 2015/6/1

N2 - Mg/Al-hydrotalcite (HDT)-dispersed paper-structured catalyst (PSC) was prepared by a simple paper-making process. The PSC exhibited excellent catalytic activity for the steam reforming of model biodiesel fuel (BDF), pure oleic acid methyl ester (oleic-FAME, C19H36O2) which is a mono-unsaturated component of practical BDFs. The PSC exhibited fuel conversion comparable to a pelletized catalyst material, here, conventional Ni-zirconia cermet anode for solid oxide fuel cell (SOFC) with less than one-hundredth Ni weight. Performance of electrolyte-supported cell connected with the PSC was evaluated in the feed of oleic-FAME, and stable operation was achieved. After 60 h test, coking was not observed in both SOFC anode and PSC.

AB - Mg/Al-hydrotalcite (HDT)-dispersed paper-structured catalyst (PSC) was prepared by a simple paper-making process. The PSC exhibited excellent catalytic activity for the steam reforming of model biodiesel fuel (BDF), pure oleic acid methyl ester (oleic-FAME, C19H36O2) which is a mono-unsaturated component of practical BDFs. The PSC exhibited fuel conversion comparable to a pelletized catalyst material, here, conventional Ni-zirconia cermet anode for solid oxide fuel cell (SOFC) with less than one-hundredth Ni weight. Performance of electrolyte-supported cell connected with the PSC was evaluated in the feed of oleic-FAME, and stable operation was achieved. After 60 h test, coking was not observed in both SOFC anode and PSC.

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