Excitation of coupled spin-orbit dynamics in cobalt oxide by femtosecond laser pulses

Takuya Satoh, Ryugo Iida, Takuya Higuchi, Yasuhiro Fujii, Akitoshi Koreeda, Hiroaki Ueda, Tsutomu Shimura, Kazuo Kuroda, V. I. Butrim, B. A. Ivanov

Research output: Contribution to journalArticle

19 Citations (Scopus)

Abstract

Ultrafast control of magnets using femtosecond light pulses attracts interest regarding applications and fundamental physics of magnetism. Antiferromagnets are promising materials with magnon frequencies extending into the terahertz range. Visible or near-infrared light interacts mainly with the electronic orbital angular momentum. In many magnets, however, in particular with iron-group ions, the orbital momentum is almost quenched by the crystal field. Thus, the interaction of magnons with light is hampered, because it is only mediated by weak unquenching of the orbital momentum by spin-orbit interactions. Here we report all-optical excitation of magnons with frequencies up to 9 THz in antiferromagnetic CoO with an unquenched orbital momentum. In CoO, magnon modes are coupled oscillations of spin and orbital momenta with comparable amplitudes. We demonstrate excitations of magnon modes by directly coupling light with electronic orbital angular momentum, providing possibilities to develop magneto-optical devices operating at several terahertz with high output-to-input ratio.

Original languageEnglish
Article number638
JournalNature communications
Volume8
Issue number1
DOIs
Publication statusPublished - Dec 1 2017

Fingerprint

cobalt oxides
Orbit
Ultrashort pulses
Momentum
Orbits
Lasers
orbits
Light
orbitals
Magnets
Angular momentum
pulses
excitation
lasers
momentum
Magnetooptical devices
Optical Devices
magnons
Photoexcitation
Physics

All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Biochemistry, Genetics and Molecular Biology(all)
  • Physics and Astronomy(all)

Cite this

Satoh, T., Iida, R., Higuchi, T., Fujii, Y., Koreeda, A., Ueda, H., ... Ivanov, B. A. (2017). Excitation of coupled spin-orbit dynamics in cobalt oxide by femtosecond laser pulses. Nature communications, 8(1), [638]. https://doi.org/10.1038/s41467-017-00616-2

Excitation of coupled spin-orbit dynamics in cobalt oxide by femtosecond laser pulses. / Satoh, Takuya; Iida, Ryugo; Higuchi, Takuya; Fujii, Yasuhiro; Koreeda, Akitoshi; Ueda, Hiroaki; Shimura, Tsutomu; Kuroda, Kazuo; Butrim, V. I.; Ivanov, B. A.

In: Nature communications, Vol. 8, No. 1, 638, 01.12.2017.

Research output: Contribution to journalArticle

Satoh, T, Iida, R, Higuchi, T, Fujii, Y, Koreeda, A, Ueda, H, Shimura, T, Kuroda, K, Butrim, VI & Ivanov, BA 2017, 'Excitation of coupled spin-orbit dynamics in cobalt oxide by femtosecond laser pulses', Nature communications, vol. 8, no. 1, 638. https://doi.org/10.1038/s41467-017-00616-2
Satoh, Takuya ; Iida, Ryugo ; Higuchi, Takuya ; Fujii, Yasuhiro ; Koreeda, Akitoshi ; Ueda, Hiroaki ; Shimura, Tsutomu ; Kuroda, Kazuo ; Butrim, V. I. ; Ivanov, B. A. / Excitation of coupled spin-orbit dynamics in cobalt oxide by femtosecond laser pulses. In: Nature communications. 2017 ; Vol. 8, No. 1.
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