As a part of an extensive study on the new geometric frustration series M2(OH)3X on deformed pyrochlore lattice, we have found an exotic antiferromagnetic order in atacamite-structure Ni2(OH)3Cl. Strong frustration exists in Ni2(OH)3Cl with antiferromagnetic transition below TN=4 K. While neutron diffraction witnessed unambiguously a long-range order, there is no signature of an order as detected by μSR. Instead, the detected local field is dynamically fluctuating at zero field. The present material may exemplify a novel type of antiferromagnetic order recently predicted for Heisenberg spins on pyrochlore lattice, wherein the squared Fourier amplitude orders but the amplitude itself fluctuates rapidly.
All Science Journal Classification (ASJC) codes
- Electronic, Optical and Magnetic Materials
- Condensed Matter Physics
- Electrical and Electronic Engineering