Facile room-temperature synthesis of highly air-stable and moisture-resistant CsPbX3/SiO2 nanocomposites for tunable white light-emitting diodes

Li Wei Chao, Jian Fu Tang, Shih Hung Lin, Yi Ting Lee, Yi Lun Chen, Cheng Ho Hsieh, Lung Chien Chen, Zong Liang Tseng

Research output: Contribution to journalArticlepeer-review

Abstract

All inorganic perovskite quantum dots (PQDs) and perovskite CsPbX3/SiO2 nanocomposites (PNCs) have shown their potentials for optical and lighting applications. We demonstrate a one-step approach to synthesize PQDs and PNCs more simply and effectively at room temperature in the open air. The resulting PNCs can show a narrow emission in the PL spectra and high stability under ambient conditions. In particular, both green CsPbBr3/SiO2 and red CsPbI3-xBrx/SiO2 PNCs can be obtained by employing this easy and low-cost method. Even, the SiO2 protection can also effectively prevent the halide exchange reaction between green and red PNCs, meaning the capability for white light applications. The resulting white light-emitting diodes (WLEDs) based on the green and red PNCs coated on the blue LED have a white Commission Internationale del’ Enclairage (CIE) coordinates of (0.375, 0.362) and a low correlated color temperature (CCT) of 4054 K.

Original languageEnglish
Article number106158
JournalMaterials Science in Semiconductor Processing
Volume136
DOIs
Publication statusPublished - Dec 2021

All Science Journal Classification (ASJC) codes

  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

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