Feasibility study of radioisotope132Cs production using accelerator-based neutrons

Md Kawchar Ahmed Patwary, Tadahiro Kin, Naoto Araki, Katsumi Aoki, Kosuke Yoshinami, Masaya Yamaguchi, Yukinobu Watanabe, Masatoshi Itoh

Research output: Contribution to journalArticle

Abstract

We propose that132Cs (Eγ = 668 keV and T1/2 = 6.5 d) can replace137Cs (Eγ = 662 keV and T1/2 = 30 y) as a new environmental tracer of cesium. The alternative tracer,132Cs, can potentially reveal the short-time dynamics in an environment, which are considered to dominate radioactive cesium absorption after nuclear accidents. We first investigate the production yield and radioactive purity of132Cs in a production experiment at the Cyclotron and Radioisotope Center of Tohoku University. The132Cs was produced via the133Cs(n,2n) reaction with neutrons generated by bombarding accelerated deuterons onto a 4 mm-thick neutron converter made of carbon. The generated neutrons were then irradiated onto a Cs2CO3 sample. The experiment yielded 102.2 kBq/g of132Cs, sufficient for tracing environmental cesium. The radioactive purity reached 98%, indicating negligible amounts of by-products. Next, a132Cs tracer experiment was performed on three different soil samples: an andosol soil, a haplic fluvisol soil, and a gleyic fluvisol soil. This feasibility study confirmed that the new tracer can measure soil cesium distributions as adequately as the137Cs tracer. Thus, we conclude that132Cs is a promising alternative environmental tracer of 137 Cs.

Original languageEnglish
Pages (from-to)280-284
Number of pages5
JournalEvergreen
Volume6
Issue number4
DOIs
Publication statusPublished - Dec 2019

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Ceramics and Composites
  • Surfaces, Coatings and Films
  • Management, Monitoring, Policy and Law

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    Patwary, M. K. A., Kin, T., Araki, N., Aoki, K., Yoshinami, K., Yamaguchi, M., Watanabe, Y., & Itoh, M. (2019). Feasibility study of radioisotope132Cs production using accelerator-based neutrons. Evergreen, 6(4), 280-284. https://doi.org/10.5109/2547352