In-plane liquid water distribution at the interface between the gas diffusion layer and catalyst layer in the cathode of a polymer electrolyte fuel cell with a hybrid pattern flow field

Hironori Nakajima, Tatsumi Kitahara, Yasutaka Takazono, Satoshi Miyahara, Akira Shimizu

Research output: Chapter in Book/Report/Conference proceedingConference contribution

1 Citation (Scopus)

Abstract

We have investigated the effect of flow field patterns without cathode humidification in a polymer electrolyte fuel cell (PEFC) using electrochemical impedance spectroscopy (EIS) with triple-parallel-serpentine, interdig-itated, and serpentine-interdigitated hybrid flow fields. The hybrid flow fields exhibit better performance than the others. The EIS results indicate that dehydration of the membrane and catalyst layer (CL) is significant for the triple-parallel-serpentine flow fields whereas that for the hybrid flow fields is not so severe. Thus the serpentine-interdigitated hybrid flow field has advantage in cell operation without cathode humidification, possibly because it provides a relatively uniform current distribution due to the in-terdigitated flow channel, and in addition, the serpentine flow channel involved in the hybrid flow field supplies water vapor along the channel. This water distribution behavior is also indicated by ex-situ tracer distribution observation using gas diffusion layers sprayed with water soluble metal salt tracer at the CL side.

Original languageEnglish
Title of host publicationPolymer Electrolyte Fuel Cells 12, PEFC 2012
Pages291-299
Number of pages9
Edition2
DOIs
Publication statusPublished - Dec 1 2012
Event12th Polymer Electrolyte Fuel Cell Symposium, PEFC 2012 - 222nd ECS Meeting - Honolulu, HI, United States
Duration: Oct 7 2012Oct 12 2012

Publication series

NameECS Transactions
Number2
Volume50
ISSN (Print)1938-5862
ISSN (Electronic)1938-6737

Other

Other12th Polymer Electrolyte Fuel Cell Symposium, PEFC 2012 - 222nd ECS Meeting
CountryUnited States
CityHonolulu, HI
Period10/7/1210/12/12

Fingerprint

Diffusion in gases
Fuel cells
Flow fields
Cathodes
Electrolytes
Catalysts
Liquids
Polymers
Water
Channel flow
Electrochemical impedance spectroscopy
Dehydration
Water vapor
Salts
Membranes
Metals

All Science Journal Classification (ASJC) codes

  • Engineering(all)

Cite this

In-plane liquid water distribution at the interface between the gas diffusion layer and catalyst layer in the cathode of a polymer electrolyte fuel cell with a hybrid pattern flow field. / Nakajima, Hironori; Kitahara, Tatsumi; Takazono, Yasutaka; Miyahara, Satoshi; Shimizu, Akira.

Polymer Electrolyte Fuel Cells 12, PEFC 2012. 2. ed. 2012. p. 291-299 (ECS Transactions; Vol. 50, No. 2).

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Nakajima, H, Kitahara, T, Takazono, Y, Miyahara, S & Shimizu, A 2012, In-plane liquid water distribution at the interface between the gas diffusion layer and catalyst layer in the cathode of a polymer electrolyte fuel cell with a hybrid pattern flow field. in Polymer Electrolyte Fuel Cells 12, PEFC 2012. 2 edn, ECS Transactions, no. 2, vol. 50, pp. 291-299, 12th Polymer Electrolyte Fuel Cell Symposium, PEFC 2012 - 222nd ECS Meeting, Honolulu, HI, United States, 10/7/12. https://doi.org/10.1149/05002.0291ecst
Nakajima, Hironori ; Kitahara, Tatsumi ; Takazono, Yasutaka ; Miyahara, Satoshi ; Shimizu, Akira. / In-plane liquid water distribution at the interface between the gas diffusion layer and catalyst layer in the cathode of a polymer electrolyte fuel cell with a hybrid pattern flow field. Polymer Electrolyte Fuel Cells 12, PEFC 2012. 2. ed. 2012. pp. 291-299 (ECS Transactions; 2).
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