Irreversible photoinduced insulator-metal transition in the Na-doped manganite (formula presented)

Takuya Satoh, Yoshinao Kikuchi, Kenjiro Miyano, Emil Pollert, Jiri Hejtmánek, Zdenek Jirák

Research output: Contribution to journalArticle

3 Citations (Scopus)

Abstract

Persistent photoconductivity has been observed in a perovskite manganite doped with an alkali metal element, (formula presented) Considering the shallow penetration depth (formula presented) of visible light, the increase of the conductance is estimated to be of the order of (formula presented) to (formula presented) which implies an irreversible photoinduced insulator-metal transition. Analysis of the dc- and ac-susceptibility data shows that the system is in a glassy state below 45 K. The system is therefore viewed as being in a highly nonuniform and metastable state, in which ferromagnetic metallic clusters exist in insulating matrix. The photoexcitation helps the clusters to dislodge from a local energy minimum and to seek more stable configuration. The percolative conduction can well explain the observed large increase of the conductivity. We argue that metastability is due to the large charge mismatch between the monovalent (formula presented) ion and (formula presented) or the incommensurability of the Mn valency from (formula presented).

Original languageEnglish
Pages (from-to)1-4
Number of pages4
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume65
Issue number12
DOIs
Publication statusPublished - Jan 1 2002
Externally publishedYes

Fingerprint

Alkali Metals
Metal insulator transition
Photoexcitation
Photoconductivity
Alkali metals
Perovskite
transition metals
insulators
Ions
metastable state
manganite
perovskite
photoexcitation
photoconductivity
alkali metals
penetration
magnetic permeability
conduction
conductivity
matrices

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

Cite this

Irreversible photoinduced insulator-metal transition in the Na-doped manganite (formula presented). / Satoh, Takuya; Kikuchi, Yoshinao; Miyano, Kenjiro; Pollert, Emil; Hejtmánek, Jiri; Jirák, Zdenek.

In: Physical Review B - Condensed Matter and Materials Physics, Vol. 65, No. 12, 01.01.2002, p. 1-4.

Research output: Contribution to journalArticle

Satoh, Takuya ; Kikuchi, Yoshinao ; Miyano, Kenjiro ; Pollert, Emil ; Hejtmánek, Jiri ; Jirák, Zdenek. / Irreversible photoinduced insulator-metal transition in the Na-doped manganite (formula presented). In: Physical Review B - Condensed Matter and Materials Physics. 2002 ; Vol. 65, No. 12. pp. 1-4.
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AU - Satoh, Takuya

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AU - Miyano, Kenjiro

AU - Pollert, Emil

AU - Hejtmánek, Jiri

AU - Jirák, Zdenek

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N2 - Persistent photoconductivity has been observed in a perovskite manganite doped with an alkali metal element, (formula presented) Considering the shallow penetration depth (formula presented) of visible light, the increase of the conductance is estimated to be of the order of (formula presented) to (formula presented) which implies an irreversible photoinduced insulator-metal transition. Analysis of the dc- and ac-susceptibility data shows that the system is in a glassy state below 45 K. The system is therefore viewed as being in a highly nonuniform and metastable state, in which ferromagnetic metallic clusters exist in insulating matrix. The photoexcitation helps the clusters to dislodge from a local energy minimum and to seek more stable configuration. The percolative conduction can well explain the observed large increase of the conductivity. We argue that metastability is due to the large charge mismatch between the monovalent (formula presented) ion and (formula presented) or the incommensurability of the Mn valency from (formula presented).

AB - Persistent photoconductivity has been observed in a perovskite manganite doped with an alkali metal element, (formula presented) Considering the shallow penetration depth (formula presented) of visible light, the increase of the conductance is estimated to be of the order of (formula presented) to (formula presented) which implies an irreversible photoinduced insulator-metal transition. Analysis of the dc- and ac-susceptibility data shows that the system is in a glassy state below 45 K. The system is therefore viewed as being in a highly nonuniform and metastable state, in which ferromagnetic metallic clusters exist in insulating matrix. The photoexcitation helps the clusters to dislodge from a local energy minimum and to seek more stable configuration. The percolative conduction can well explain the observed large increase of the conductivity. We argue that metastability is due to the large charge mismatch between the monovalent (formula presented) ion and (formula presented) or the incommensurability of the Mn valency from (formula presented).

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