Low-temperature synthesis of high-purity single-walled carbon nanotubes from alcohol

Shigeo Maruyama, Ryosuke Kojima, Yuhei Miyauchi, Shohei Chiashi, Masamichi Kohno

Research output: Contribution to journalArticle

896 Citations (Scopus)

Abstract

By using alcohol as the carbon source, a new simple catalytic chemical vapor deposition technique to synthesize high-purity single-walled carbon nanotubes at low temperature is demonstrated. Because of the etching effect of decomposed OH radical attacking carbon atoms with a dangling bond, impurities such as amorphous carbon, multi-walled carbon nanotubes, metal particles and carbon nanoparticles are completely suppressed even at relatively low reaction temperature such as 700-800 °C. By using methanol, generation of SWNTs even at 550 °C is demonstrated. The high-purity synthesis at low temperature promises large scale production at low cost and the direct growth of SWNTs on conventional semiconductor devices already patterned with aluminum.

Original languageEnglish
Pages (from-to)229-234
Number of pages6
JournalChemical Physics Letters
Volume360
Issue number3-4
DOIs
Publication statusPublished - Jul 10 2002
Externally publishedYes

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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