Magnetic properties of Haldane system TMNIN of finite chain length

Tatsuya Kawae, M. Ito, M. Mito, M. Hitaka, K. Takeda

Research output: Contribution to journalArticle

Abstract

We have studied magnetic properties ofa Haldane system antiferromagnet (CH3)4NNi(NO)3 (TMNIN) diluted with nonmagnetic impurity Zn 2+ ions for the concentration, 7.0 %, 11.4 % and 20.4 % as well as non-diluted system. The susceptibility shows the Curie-law attributed to the edge spins of one-dimensional chain down to 1 K with tile Curie constant of 40 % of that expected of the free spin in the case of the VBS model. At lower temperature than 1 K, however, the paramagnetic contribution is found to be suppressed for the higher concentrations. In the heat capacity measurements: a small bump is observed around 0.6 K. The present results suggest the existence of the magnetic interaction between the edge spins via Zn 2+ ions or between the edge spins within 1D chain.

Original languageEnglish
Pages (from-to)1935-1936
Number of pages2
JournalCzechoslovak Journal of Physics
Volume46
Issue numberSUPPL. 4
DOIs
Publication statusPublished - Dec 1 1996

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magnetic properties
tiles
ions
specific heat
magnetic permeability
impurities
interactions

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)

Cite this

Magnetic properties of Haldane system TMNIN of finite chain length. / Kawae, Tatsuya; Ito, M.; Mito, M.; Hitaka, M.; Takeda, K.

In: Czechoslovak Journal of Physics, Vol. 46, No. SUPPL. 4, 01.12.1996, p. 1935-1936.

Research output: Contribution to journalArticle

Kawae, Tatsuya ; Ito, M. ; Mito, M. ; Hitaka, M. ; Takeda, K. / Magnetic properties of Haldane system TMNIN of finite chain length. In: Czechoslovak Journal of Physics. 1996 ; Vol. 46, No. SUPPL. 4. pp. 1935-1936.
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