Molecular frame image restoration and partial wave analysis of photoionization dynamics of NO by time-energy mapping of photoelectron angular distribution

Ying Tang, Yoshi Ichi Suzuki, Takuya Horio, Toshinori Suzuki

Research output: Contribution to journalArticle

27 Citations (Scopus)

Abstract

The benchmark system of molecular photoionization dynamics, the (1+1 ) two-photon ionization of NO via the A state, is investigated using the time-energy mapping of the photoelectron angular distribution in a laboratory frame. The molecular frame photoelectron angular distribution and partial wave composition are determined from time-energy maps and compared with those obtained by Schwinger variational calculation (SVC) and state-to-state photoelectron spectroscopy. Good agreement is found with SVC. By comparison of the phase shifts of the scattering waves and the quantum defects of the Rydberg states, the l hybridization of p waves is identified.

Original languageEnglish
Article number073002
JournalPhysical Review Letters
Volume104
Issue number7
DOIs
Publication statusPublished - Feb 17 2010

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restoration
photoionization
photoelectrons
angular distribution
wave scattering
phase shift
photoelectron spectroscopy
ionization
energy
defects
photons

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)

Cite this

Molecular frame image restoration and partial wave analysis of photoionization dynamics of NO by time-energy mapping of photoelectron angular distribution. / Tang, Ying; Suzuki, Yoshi Ichi; Horio, Takuya; Suzuki, Toshinori.

In: Physical Review Letters, Vol. 104, No. 7, 073002, 17.02.2010.

Research output: Contribution to journalArticle

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