Numerical analysis of effects of electric field and pulse duration on discharge DeNoX performance

Kohei Ito, Katuyuki Hagiwara, Hiroyuki Nakaura, Kazuo Onda, Hidekazu Tanaka

Research output: Contribution to journalArticle

2 Citations (Scopus)

Abstract

By virtue of its comparatively high denitrification (deNOx) efficiency and its compactness, the pulsed-discharge deNOx process is considered to be one of the deNOx processes suitable for combustion gas. However, there has been insufficient clear guidance on the optimum electric field, pulse duration, and pulse repetition frequency, and no clear understanding of pulsed-discharge deNOx process. In this study, we have simulated the pulsed-discharge deNOx process by solving the Boltzmann equation for discharge electrons and the deNOx chemical reaction equations simultaneously, and we have shown the time change of chemical species concentration, extracting the main deNOx reactions. The simulation shows that the pulsed-discharge deNOx process consists of two processes, the reduction of NO to N2 by N radicals and the oxidation of NO to HNO3 and HNO2 by OH and O radicals, and that the amounts of radicals produced and consumed are governed by parameters such as the electric field, pulse duration, and pulse repetition frequency. In our simulation, such parameters are varied widely to examine their quantitative effect on the deNOx energy consumption, NxOy removal efficiency, and reduction ratio in the discharge deNOx process. The preliminary pulsed-discharge deNOx performance is estimated from our simulation, indicating that the discharge deNOx process has almost the same performance as the electron-beam deNOx process.

Original languageEnglish
Pages (from-to)1-11
Number of pages11
JournalElectrical Engineering in Japan (English translation of Denki Gakkai Ronbunshi)
Volume139
Issue number2
DOIs
Publication statusPublished - Apr 30 2002

Fingerprint

Numerical analysis
Electric fields
Boltzmann equation
Denitrification
Chemical reactions
Electron beams
Energy utilization
Oxidation
Electrons
Gases

All Science Journal Classification (ASJC) codes

  • Energy Engineering and Power Technology
  • Electrical and Electronic Engineering

Cite this

Numerical analysis of effects of electric field and pulse duration on discharge DeNoX performance. / Ito, Kohei; Hagiwara, Katuyuki; Nakaura, Hiroyuki; Onda, Kazuo; Tanaka, Hidekazu.

In: Electrical Engineering in Japan (English translation of Denki Gakkai Ronbunshi), Vol. 139, No. 2, 30.04.2002, p. 1-11.

Research output: Contribution to journalArticle

@article{ec80c9bfbc3a4f9eb5eefc017d952bc9,
title = "Numerical analysis of effects of electric field and pulse duration on discharge DeNoX performance",
abstract = "By virtue of its comparatively high denitrification (deNOx) efficiency and its compactness, the pulsed-discharge deNOx process is considered to be one of the deNOx processes suitable for combustion gas. However, there has been insufficient clear guidance on the optimum electric field, pulse duration, and pulse repetition frequency, and no clear understanding of pulsed-discharge deNOx process. In this study, we have simulated the pulsed-discharge deNOx process by solving the Boltzmann equation for discharge electrons and the deNOx chemical reaction equations simultaneously, and we have shown the time change of chemical species concentration, extracting the main deNOx reactions. The simulation shows that the pulsed-discharge deNOx process consists of two processes, the reduction of NO to N2 by N radicals and the oxidation of NO to HNO3 and HNO2 by OH and O radicals, and that the amounts of radicals produced and consumed are governed by parameters such as the electric field, pulse duration, and pulse repetition frequency. In our simulation, such parameters are varied widely to examine their quantitative effect on the deNOx energy consumption, NxOy removal efficiency, and reduction ratio in the discharge deNOx process. The preliminary pulsed-discharge deNOx performance is estimated from our simulation, indicating that the discharge deNOx process has almost the same performance as the electron-beam deNOx process.",
author = "Kohei Ito and Katuyuki Hagiwara and Hiroyuki Nakaura and Kazuo Onda and Hidekazu Tanaka",
year = "2002",
month = "4",
day = "30",
doi = "10.1002/eej.1149",
language = "English",
volume = "139",
pages = "1--11",
journal = "Electrical Engineering in Japan (English translation of Denki Gakkai Ronbunshi)",
issn = "0424-7760",
publisher = "John Wiley and Sons Inc.",
number = "2",

}

TY - JOUR

T1 - Numerical analysis of effects of electric field and pulse duration on discharge DeNoX performance

AU - Ito, Kohei

AU - Hagiwara, Katuyuki

AU - Nakaura, Hiroyuki

AU - Onda, Kazuo

AU - Tanaka, Hidekazu

PY - 2002/4/30

Y1 - 2002/4/30

N2 - By virtue of its comparatively high denitrification (deNOx) efficiency and its compactness, the pulsed-discharge deNOx process is considered to be one of the deNOx processes suitable for combustion gas. However, there has been insufficient clear guidance on the optimum electric field, pulse duration, and pulse repetition frequency, and no clear understanding of pulsed-discharge deNOx process. In this study, we have simulated the pulsed-discharge deNOx process by solving the Boltzmann equation for discharge electrons and the deNOx chemical reaction equations simultaneously, and we have shown the time change of chemical species concentration, extracting the main deNOx reactions. The simulation shows that the pulsed-discharge deNOx process consists of two processes, the reduction of NO to N2 by N radicals and the oxidation of NO to HNO3 and HNO2 by OH and O radicals, and that the amounts of radicals produced and consumed are governed by parameters such as the electric field, pulse duration, and pulse repetition frequency. In our simulation, such parameters are varied widely to examine their quantitative effect on the deNOx energy consumption, NxOy removal efficiency, and reduction ratio in the discharge deNOx process. The preliminary pulsed-discharge deNOx performance is estimated from our simulation, indicating that the discharge deNOx process has almost the same performance as the electron-beam deNOx process.

AB - By virtue of its comparatively high denitrification (deNOx) efficiency and its compactness, the pulsed-discharge deNOx process is considered to be one of the deNOx processes suitable for combustion gas. However, there has been insufficient clear guidance on the optimum electric field, pulse duration, and pulse repetition frequency, and no clear understanding of pulsed-discharge deNOx process. In this study, we have simulated the pulsed-discharge deNOx process by solving the Boltzmann equation for discharge electrons and the deNOx chemical reaction equations simultaneously, and we have shown the time change of chemical species concentration, extracting the main deNOx reactions. The simulation shows that the pulsed-discharge deNOx process consists of two processes, the reduction of NO to N2 by N radicals and the oxidation of NO to HNO3 and HNO2 by OH and O radicals, and that the amounts of radicals produced and consumed are governed by parameters such as the electric field, pulse duration, and pulse repetition frequency. In our simulation, such parameters are varied widely to examine their quantitative effect on the deNOx energy consumption, NxOy removal efficiency, and reduction ratio in the discharge deNOx process. The preliminary pulsed-discharge deNOx performance is estimated from our simulation, indicating that the discharge deNOx process has almost the same performance as the electron-beam deNOx process.

UR - http://www.scopus.com/inward/record.url?scp=0037197597&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=0037197597&partnerID=8YFLogxK

U2 - 10.1002/eej.1149

DO - 10.1002/eej.1149

M3 - Article

VL - 139

SP - 1

EP - 11

JO - Electrical Engineering in Japan (English translation of Denki Gakkai Ronbunshi)

JF - Electrical Engineering in Japan (English translation of Denki Gakkai Ronbunshi)

SN - 0424-7760

IS - 2

ER -