Platinum nanoparticles supported on reduced graphene oxide prepared in situ by a continuous one-step laser process

Ina Haxhiaj, Sebastian Tigges, Damian Firla, Xiaorui Zhang, Ulrich Hagemann, Takahiro Kondo, Junji Nakamura, Galina Marzun, Stephan Barcikowski

Research output: Contribution to journalArticlepeer-review

18 Citations (Scopus)

Abstract

A large research emphasis is still placed on improvement of production routes of nanosized materials with enhanced catalytic properties. Here we developed a continuous process for generation of platinum (Pt) nanoparticles supported on reduced graphene oxide (rGO) in situ via pulsed laser ablation in liquid (PLAL) dispersion of rGO. This in situ PLAL technique is a single step procedure that allows the synthesis of heterogeneous catalysts with a simultaneous control of particle size and mass loading. By this method, Pt particles with mean particle diameters around 2.5 nm and in a regime of 3–4 nm have been produced in ethanol and saline water, respectively, and adsorbed on rGO with up to 50 wt%. Both inorganic and organic solvents used during in situ synthesis lead to production of CO tolerant Pt/rGO catalysts, which are relevant for fuel cell applications due to the remarkably low CO desorption temperatures around 65–80 °C.

Original languageEnglish
Pages (from-to)811-820
Number of pages10
JournalApplied Surface Science
Volume469
DOIs
Publication statusPublished - Mar 1 2019
Externally publishedYes

All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Condensed Matter Physics
  • Physics and Astronomy(all)
  • Surfaces and Interfaces
  • Surfaces, Coatings and Films

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