Preliminary study on catalytic combustion-type sensor for the detection of diesel particulate matter

Cheol Beom Lim; Hisahiro Einaga; Yoshihiko Sadaoka; Yasutake Teraoka

doi:10.1016/j.snb.2011.08.009

Preliminary study on catalytic combustion-type sensor for the detection of diesel particulate matter

Cheol Beom Lim, Hisahiro Einaga, Yoshihiko Sadaoka, Yasutake Teraoka

Functional Materials Science

Research output: Contribution to journal › Article › peer-review

13 Citations (Scopus)

Abstract

Catalytic oxidation and sensing of simulated diesel particulate matter (PM), which consists of hexadecane and carbon black as substitutes of soluble organic fraction (SOF) and soot, respectively, were investigated with Ag and Pt catalysts supported on TiO₂ and CeO₂. Supported Ag catalysts were active for soot oxidation at temperatures over about 500 °C, while supported Pt catalysts were almost inactive for the soot oxidation. Toward the oxidation of SOF, on the other hand, supported Pt catalysts were more active than supported Ag catalysts. Catalytic combustion-type sensors coated with those catalysts was fabricated, and their sensing characteristics were evaluated. Because of the difficulty to simulate the real sensing condition of PM, employed in this study was the programmed heating of the sensor on which PM or soot was pre-loaded. The results strongly suggest the possibilities to construct the catalytic combustion-type PM sensor and to selectively detect SOF and soot by the proper selection of the catalytic materials and operation temperatures.

Original language	English
Pages (from-to)	463-470
Number of pages	8
Journal	Sensors and Actuators, B: Chemical
Volume	160
Issue number	1
DOIs	https://doi.org/10.1016/j.snb.2011.08.009
Publication status	Published - Dec 15 2011

All Science Journal Classification (ASJC) codes

Electronic, Optical and Magnetic Materials
Instrumentation
Condensed Matter Physics
Surfaces, Coatings and Films
Metals and Alloys
Electrical and Electronic Engineering
Materials Chemistry

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title = "Preliminary study on catalytic combustion-type sensor for the detection of diesel particulate matter",

abstract = "Catalytic oxidation and sensing of simulated diesel particulate matter (PM), which consists of hexadecane and carbon black as substitutes of soluble organic fraction (SOF) and soot, respectively, were investigated with Ag and Pt catalysts supported on TiO2 and CeO2. Supported Ag catalysts were active for soot oxidation at temperatures over about 500 °C, while supported Pt catalysts were almost inactive for the soot oxidation. Toward the oxidation of SOF, on the other hand, supported Pt catalysts were more active than supported Ag catalysts. Catalytic combustion-type sensors coated with those catalysts was fabricated, and their sensing characteristics were evaluated. Because of the difficulty to simulate the real sensing condition of PM, employed in this study was the programmed heating of the sensor on which PM or soot was pre-loaded. The results strongly suggest the possibilities to construct the catalytic combustion-type PM sensor and to selectively detect SOF and soot by the proper selection of the catalytic materials and operation temperatures.",

author = "Lim, {Cheol Beom} and Hisahiro Einaga and Yoshihiko Sadaoka and Yasutake Teraoka",

note = "Funding Information: The author (C.B. Lim) is grateful for financial assistance provided by the Global-Centre of Excellence in Novel Carbon Resource Sciences, Kyushu University . ",

year = "2011",

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doi = "10.1016/j.snb.2011.08.009",

language = "English",

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T1 - Preliminary study on catalytic combustion-type sensor for the detection of diesel particulate matter

AU - Lim, Cheol Beom

AU - Einaga, Hisahiro

AU - Sadaoka, Yoshihiko

AU - Teraoka, Yasutake

N1 - Funding Information: The author (C.B. Lim) is grateful for financial assistance provided by the Global-Centre of Excellence in Novel Carbon Resource Sciences, Kyushu University .

PY - 2011/12/15

Y1 - 2011/12/15

N2 - Catalytic oxidation and sensing of simulated diesel particulate matter (PM), which consists of hexadecane and carbon black as substitutes of soluble organic fraction (SOF) and soot, respectively, were investigated with Ag and Pt catalysts supported on TiO2 and CeO2. Supported Ag catalysts were active for soot oxidation at temperatures over about 500 °C, while supported Pt catalysts were almost inactive for the soot oxidation. Toward the oxidation of SOF, on the other hand, supported Pt catalysts were more active than supported Ag catalysts. Catalytic combustion-type sensors coated with those catalysts was fabricated, and their sensing characteristics were evaluated. Because of the difficulty to simulate the real sensing condition of PM, employed in this study was the programmed heating of the sensor on which PM or soot was pre-loaded. The results strongly suggest the possibilities to construct the catalytic combustion-type PM sensor and to selectively detect SOF and soot by the proper selection of the catalytic materials and operation temperatures.

AB - Catalytic oxidation and sensing of simulated diesel particulate matter (PM), which consists of hexadecane and carbon black as substitutes of soluble organic fraction (SOF) and soot, respectively, were investigated with Ag and Pt catalysts supported on TiO2 and CeO2. Supported Ag catalysts were active for soot oxidation at temperatures over about 500 °C, while supported Pt catalysts were almost inactive for the soot oxidation. Toward the oxidation of SOF, on the other hand, supported Pt catalysts were more active than supported Ag catalysts. Catalytic combustion-type sensors coated with those catalysts was fabricated, and their sensing characteristics were evaluated. Because of the difficulty to simulate the real sensing condition of PM, employed in this study was the programmed heating of the sensor on which PM or soot was pre-loaded. The results strongly suggest the possibilities to construct the catalytic combustion-type PM sensor and to selectively detect SOF and soot by the proper selection of the catalytic materials and operation temperatures.

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Preliminary study on catalytic combustion-type sensor for the detection of diesel particulate matter

Abstract

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