Production of high-purity medical radio isotope 64Cu with accelerator-based neutrons generated with 9 and 12 MeV deuterons

Tadahiro Kin, Takaya Kawagoe, Shouhei Araki, Yukinobu Watanabe

Research output: Contribution to journalArticle

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Abstract

We conducted a feasibility study for producing a high-purity medical radioisotope 64Cu from natural zinc with accelerator-based neutrons. 64Cu isotopes were produced via the 64Zn(n,p) reaction. The accelerator-based neutrons were generated via the C(d,n) reaction using low-energy deuterons of 9 and 12 MeV on a 1-mm-thick carbon target. First, the production purity was estimated using the evaluated nuclear data library JENDL-4.0 and our previously measured thick target neutron yield. We found that even when natural zinc was used as the starting material, significantly high-purity 64Cu could be obtained. Next, irradiation experiments for producing 64Cu using natural zinc were conducted at Kyushu University Tandem Laboratory, with the amounts of 64Cu isotopes and other gamma-emission nuclides measured by a high-purity germanium detector. As a result, high-purity 64Cu isotopes of 1.11(49) × 100 and 3.70 (17) × 100 Bq/g/C were produced with incident deuteron energies of 9 and 12 MeV, respectively.

Original languageEnglish
Pages (from-to)1123-1130
Number of pages8
Journaljournal of nuclear science and technology
Volume54
Issue number10
DOIs
Publication statusPublished - Oct 3 2017

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Isotopes
Particle accelerators
deuterons
Neutrons
purity
accelerators
isotopes
neutrons
Zinc
zinc
Germanium
Radioisotopes
nuclides
Irradiation
germanium
Detectors
Carbon
irradiation
energy
carbon

All Science Journal Classification (ASJC) codes

  • Nuclear and High Energy Physics
  • Nuclear Energy and Engineering

Cite this

Production of high-purity medical radio isotope 64Cu with accelerator-based neutrons generated with 9 and 12 MeV deuterons. / Kin, Tadahiro; Kawagoe, Takaya; Araki, Shouhei; Watanabe, Yukinobu.

In: journal of nuclear science and technology, Vol. 54, No. 10, 03.10.2017, p. 1123-1130.

Research output: Contribution to journalArticle

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AB - We conducted a feasibility study for producing a high-purity medical radioisotope 64Cu from natural zinc with accelerator-based neutrons. 64Cu isotopes were produced via the 64Zn(n,p) reaction. The accelerator-based neutrons were generated via the C(d,n) reaction using low-energy deuterons of 9 and 12 MeV on a 1-mm-thick carbon target. First, the production purity was estimated using the evaluated nuclear data library JENDL-4.0 and our previously measured thick target neutron yield. We found that even when natural zinc was used as the starting material, significantly high-purity 64Cu could be obtained. Next, irradiation experiments for producing 64Cu using natural zinc were conducted at Kyushu University Tandem Laboratory, with the amounts of 64Cu isotopes and other gamma-emission nuclides measured by a high-purity germanium detector. As a result, high-purity 64Cu isotopes of 1.11(49) × 100 and 3.70 (17) × 100 Bq/g/C were produced with incident deuteron energies of 9 and 12 MeV, respectively.

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