Real-time observational evidence of changing Asian dust morphology with the mixing of heavy anthropogenic pollution

Xiaole Pan, Itsushi Uno, Zhe Wang, Tomoaki Nishizawa, Nobuo Sugimoto, Shigekazu Yamamoto, Hiroshi Kobayashi, Yele Sun, Pingqing Fu, Xiao Tang, Zifa Wang

Research output: Contribution to journalArticle

33 Citations (Scopus)

Abstract

Natural mineral dust and heavy anthropogenic pollution and its complex interactions cause significant environmental problems in East Asia. Due to restrictions of observing technique, real-time morphological change in Asian dust particles owing to coating process of anthropogenic pollutants is still statistically unclear. Here, we first used a newly developed, single-particle polarization detector and quantitatively investigate the evolution of the polarization property of backscattering light reflected from dust particle as they were mixing with anthropogenic pollutants in North China. The decrease in observed depolarization ratio is mainly attributed to the decrease of aspect ratio of the dust particles as a result of continuous coating processes. Hygroscopic growth of Calcium nitrate (Ca(NO3)2) on the surface of the dust particles played a vital role, particularly when they are stagnant in the polluted region with high RH conditions. Reliable statistics highlight the significant importance of internally mixed, 'quasi-spherical' Asian dust particles, which markedly act as cloud condensation nuclei and exert regional climate change.

Original languageEnglish
Article number335
JournalScientific reports
Volume7
Issue number1
DOIs
Publication statusPublished - Dec 1 2017

All Science Journal Classification (ASJC) codes

  • General

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