Real-time spectroscopy of Frenkel exciton system

Hideaki Kano, Takayoshi Kobayashi

Research output: Contribution to journalArticlepeer-review

9 Citations (Scopus)

Abstract

We performed selective excitations of the first- and second-excited Frenkel exciton states (Q- and B-excitons) with use of sub-40-fs and sub-5-fs visible laser pulses. The transient absorption signals exhibit oscillatory features associated with molecular vibrations. From an analysis of the spectral profiles of the phase and amplitude of the oscillation, the experimental result is well explained by the modulated transition dipole moment, which is caused by the dynamic intensity borrowing from the intense B-transition to the weak Q-transition.

Original languageEnglish
Pages (from-to)269-282
Number of pages14
JournalJournal of Luminescence
Volume100
Issue number1-4
DOIs
Publication statusPublished - Dec 2002
Externally publishedYes

All Science Journal Classification (ASJC) codes

  • Biophysics
  • Biochemistry
  • Chemistry(all)
  • Atomic and Molecular Physics, and Optics
  • Condensed Matter Physics

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