Spallation reaction study for the long-lived fission product 107 Pd

He Wang, Hideaki Otsu, Hiroyoshi Sakurai, Deuksoon Ahn, Masayuki Aikawa, Takashi Ando, Shouhei Araki, Sidong Chen, Nobuyuki Chiga, Pieter Doornenbal, Naoki Fukuda, Tadaaki Isobe, Shunsuke Kawakami, Shoichiro Kawase, Tadahiro Kin, Yosuke Kondo, Shunpei Koyama, Shigeru Kubono, Yukie Maeda, Ayano Makinaga & 29 others Masafumi Matsushita, Teiichiro Matsuzaki, Shin'Ichiro Michimasa, Satoru Momiyama, Shunsuke Nagamine, Takashi Nakamura, Keita Nakano, Megumi Niikura, Tomoyuki Ozaki, Atsumi Saito, Takeshi Saito, Yoshiaki Shiga, Mizuki Shikata, Yohei Shimizu, Susumu Shimoura, Toshiyuki Sumikama, Pär Anders Söderström, Hiroshi Suzuki, Hiroyuki Takeda, Satoshi Takeuchi, Ryo Taniuchi, Yasuhiro Togano, Junichi Tsubota, Meiko Uesaka, Yasushi Watanabe, Yukinobu Watanabe, Kathrin Wimmer, Tatsuya Yamamoto, Koichi Yoshida

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Abstract

Spallation reactions for the long-lived fission product 107Pd have been studied for the purpose of nuclear waste transmutation. The cross sections on the proton- and deuteron-induced spallation were obtained at 196 and 118 MeV/nucleon in inverse kinematics at the RIKEN Radioactive Isotope Beam Factory. Both the target and energy dependences of cross sections have been investigated systematically. It was found that the proton-induced cross sections at 196 MeV/nucleon are close to those for deuteron obtained at 118 MeV/nucleon for the light-mass products. The experimental data are compared with the SPACS semi-empirical parameterization and the PHITS calculations including both the intranuclear cascade and evaporation processes. Our data give a design goal of proton/deuteron flux for the transmutation of 107 Pd using the spallation reaction. In addition, it is found that the spallation reaction at 118 MeV/nucleon may have an advantage over the 107 Pd transmutation because of the low production of other long-lived radioactive isotopes.

Original languageEnglish
Article number021D01
JournalProgress of Theoretical and Experimental Physics
Volume2017
Issue number2
DOIs
Publication statusPublished - Feb 1 2017

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fission products
spallation
transmutation
deuterons
radioactive isotopes
protons
cross sections
inverse kinematics
radioactive wastes
industrial plants
parameterization
cascades
evaporation
products
energy

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)

Cite this

Wang, H., Otsu, H., Sakurai, H., Ahn, D., Aikawa, M., Ando, T., ... Yoshida, K. (2017). Spallation reaction study for the long-lived fission product 107 Pd Progress of Theoretical and Experimental Physics, 2017(2), [021D01]. https://doi.org/10.1093/ptep/ptw187

Spallation reaction study for the long-lived fission product 107 Pd . / Wang, He; Otsu, Hideaki; Sakurai, Hiroyoshi; Ahn, Deuksoon; Aikawa, Masayuki; Ando, Takashi; Araki, Shouhei; Chen, Sidong; Chiga, Nobuyuki; Doornenbal, Pieter; Fukuda, Naoki; Isobe, Tadaaki; Kawakami, Shunsuke; Kawase, Shoichiro; Kin, Tadahiro; Kondo, Yosuke; Koyama, Shunpei; Kubono, Shigeru; Maeda, Yukie; Makinaga, Ayano; Matsushita, Masafumi; Matsuzaki, Teiichiro; Michimasa, Shin'Ichiro; Momiyama, Satoru; Nagamine, Shunsuke; Nakamura, Takashi; Nakano, Keita; Niikura, Megumi; Ozaki, Tomoyuki; Saito, Atsumi; Saito, Takeshi; Shiga, Yoshiaki; Shikata, Mizuki; Shimizu, Yohei; Shimoura, Susumu; Sumikama, Toshiyuki; Söderström, Pär Anders; Suzuki, Hiroshi; Takeda, Hiroyuki; Takeuchi, Satoshi; Taniuchi, Ryo; Togano, Yasuhiro; Tsubota, Junichi; Uesaka, Meiko; Watanabe, Yasushi; Watanabe, Yukinobu; Wimmer, Kathrin; Yamamoto, Tatsuya; Yoshida, Koichi.

In: Progress of Theoretical and Experimental Physics, Vol. 2017, No. 2, 021D01, 01.02.2017.

Research output: Contribution to journalArticle

Wang, H, Otsu, H, Sakurai, H, Ahn, D, Aikawa, M, Ando, T, Araki, S, Chen, S, Chiga, N, Doornenbal, P, Fukuda, N, Isobe, T, Kawakami, S, Kawase, S, Kin, T, Kondo, Y, Koyama, S, Kubono, S, Maeda, Y, Makinaga, A, Matsushita, M, Matsuzaki, T, Michimasa, SI, Momiyama, S, Nagamine, S, Nakamura, T, Nakano, K, Niikura, M, Ozaki, T, Saito, A, Saito, T, Shiga, Y, Shikata, M, Shimizu, Y, Shimoura, S, Sumikama, T, Söderström, PA, Suzuki, H, Takeda, H, Takeuchi, S, Taniuchi, R, Togano, Y, Tsubota, J, Uesaka, M, Watanabe, Y, Watanabe, Y, Wimmer, K, Yamamoto, T & Yoshida, K 2017, ' Spallation reaction study for the long-lived fission product 107 Pd ', Progress of Theoretical and Experimental Physics, vol. 2017, no. 2, 021D01. https://doi.org/10.1093/ptep/ptw187
Wang, He ; Otsu, Hideaki ; Sakurai, Hiroyoshi ; Ahn, Deuksoon ; Aikawa, Masayuki ; Ando, Takashi ; Araki, Shouhei ; Chen, Sidong ; Chiga, Nobuyuki ; Doornenbal, Pieter ; Fukuda, Naoki ; Isobe, Tadaaki ; Kawakami, Shunsuke ; Kawase, Shoichiro ; Kin, Tadahiro ; Kondo, Yosuke ; Koyama, Shunpei ; Kubono, Shigeru ; Maeda, Yukie ; Makinaga, Ayano ; Matsushita, Masafumi ; Matsuzaki, Teiichiro ; Michimasa, Shin'Ichiro ; Momiyama, Satoru ; Nagamine, Shunsuke ; Nakamura, Takashi ; Nakano, Keita ; Niikura, Megumi ; Ozaki, Tomoyuki ; Saito, Atsumi ; Saito, Takeshi ; Shiga, Yoshiaki ; Shikata, Mizuki ; Shimizu, Yohei ; Shimoura, Susumu ; Sumikama, Toshiyuki ; Söderström, Pär Anders ; Suzuki, Hiroshi ; Takeda, Hiroyuki ; Takeuchi, Satoshi ; Taniuchi, Ryo ; Togano, Yasuhiro ; Tsubota, Junichi ; Uesaka, Meiko ; Watanabe, Yasushi ; Watanabe, Yukinobu ; Wimmer, Kathrin ; Yamamoto, Tatsuya ; Yoshida, Koichi. / Spallation reaction study for the long-lived fission product 107 Pd In: Progress of Theoretical and Experimental Physics. 2017 ; Vol. 2017, No. 2.
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abstract = "Spallation reactions for the long-lived fission product 107Pd have been studied for the purpose of nuclear waste transmutation. The cross sections on the proton- and deuteron-induced spallation were obtained at 196 and 118 MeV/nucleon in inverse kinematics at the RIKEN Radioactive Isotope Beam Factory. Both the target and energy dependences of cross sections have been investigated systematically. It was found that the proton-induced cross sections at 196 MeV/nucleon are close to those for deuteron obtained at 118 MeV/nucleon for the light-mass products. The experimental data are compared with the SPACS semi-empirical parameterization and the PHITS calculations including both the intranuclear cascade and evaporation processes. Our data give a design goal of proton/deuteron flux for the transmutation of 107 Pd using the spallation reaction. In addition, it is found that the spallation reaction at 118 MeV/nucleon may have an advantage over the 107 Pd transmutation because of the low production of other long-lived radioactive isotopes.",
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AU - Ando, Takashi

AU - Araki, Shouhei

AU - Chen, Sidong

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AU - Matsuzaki, Teiichiro

AU - Michimasa, Shin'Ichiro

AU - Momiyama, Satoru

AU - Nagamine, Shunsuke

AU - Nakamura, Takashi

AU - Nakano, Keita

AU - Niikura, Megumi

AU - Ozaki, Tomoyuki

AU - Saito, Atsumi

AU - Saito, Takeshi

AU - Shiga, Yoshiaki

AU - Shikata, Mizuki

AU - Shimizu, Yohei

AU - Shimoura, Susumu

AU - Sumikama, Toshiyuki

AU - Söderström, Pär Anders

AU - Suzuki, Hiroshi

AU - Takeda, Hiroyuki

AU - Takeuchi, Satoshi

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AU - Tsubota, Junichi

AU - Uesaka, Meiko

AU - Watanabe, Yasushi

AU - Watanabe, Yukinobu

AU - Wimmer, Kathrin

AU - Yamamoto, Tatsuya

AU - Yoshida, Koichi

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