Statistical estimate of mercury removal efficiencies for air pollution control devices of municipal solid waste incinerators

Fumitake Takahashi, Akiko Kida, Takayuki Shimaoka

Research output: Contribution to journalArticle

16 Citations (Scopus)

Abstract

Although representative removal efficiencies of gaseous mercury for air pollution control devices (APCDs) are important to prepare more reliable atmospheric emission inventories of mercury, they have been still uncertain because they depend sensitively on many factors like the type of APCDs, gas temperature, and mercury speciation. In this study, representative removal efficiencies of gaseous mercury for several types of APCDs of municipal solid waste incineration (MSWI) were offered using a statistical method. 534 data of mercury removal efficiencies for APCDs used in MSWI were collected. APCDs were categorized as fixed-bed absorber (FA), wet scrubber (WS), electrostatic precipitator (ESP), and fabric filter (FF), and their hybrid systems. Data series of all APCD types had Gaussian log-normality. The average removal efficiency with a 95% confidence interval for each APCD was estimated. The FA, WS, and FF with carbon and/or dry sorbent injection systems had 75% to 82% average removal efficiencies. On the other hand, the ESP with/without dry sorbent injection had lower removal efficiencies of up to 22%. The type of dry sorbent injection in the FF system, dry or semi-dry, did not make more than 1% difference to the removal efficiency. The injection of activated carbon and carbon-containing fly ash in the FF system made less than 3% difference. Estimation errors of removal efficiency were especially high for the ESP. The national average of removal efficiency of APCDs in Japanese MSWI plants was estimated on the basis of incineration capacity. Owing to the replacement of old APCDs for dioxin control, the national average removal efficiency increased from 34.5% in 1991 to 92.5% in 2003. This resulted in an additional reduction of about 0.86. Mg emission in 2003. Further study using the methodology in this study to other important emission sources like coal-fired power plants will contribute to better emission inventories.

Original languageEnglish
Pages (from-to)5472-5477
Number of pages6
JournalScience of the Total Environment
Volume408
Issue number22
DOIs
Publication statusPublished - Oct 1 2010

Fingerprint

Air pollution control
Refuse incinerators
Municipal solid waste
Mercury
municipal solid waste
pollution control
atmospheric pollution
Waste incineration
incineration
Electrostatic precipitators
Sorbents
filter
Scrubbers
emission inventory
Carbon
mercury
removal
waste incinerator
Coal Ash
Dioxins

All Science Journal Classification (ASJC) codes

  • Environmental Engineering
  • Environmental Chemistry
  • Waste Management and Disposal
  • Pollution

Cite this

Statistical estimate of mercury removal efficiencies for air pollution control devices of municipal solid waste incinerators. / Takahashi, Fumitake; Kida, Akiko; Shimaoka, Takayuki.

In: Science of the Total Environment, Vol. 408, No. 22, 01.10.2010, p. 5472-5477.

Research output: Contribution to journalArticle

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abstract = "Although representative removal efficiencies of gaseous mercury for air pollution control devices (APCDs) are important to prepare more reliable atmospheric emission inventories of mercury, they have been still uncertain because they depend sensitively on many factors like the type of APCDs, gas temperature, and mercury speciation. In this study, representative removal efficiencies of gaseous mercury for several types of APCDs of municipal solid waste incineration (MSWI) were offered using a statistical method. 534 data of mercury removal efficiencies for APCDs used in MSWI were collected. APCDs were categorized as fixed-bed absorber (FA), wet scrubber (WS), electrostatic precipitator (ESP), and fabric filter (FF), and their hybrid systems. Data series of all APCD types had Gaussian log-normality. The average removal efficiency with a 95{\%} confidence interval for each APCD was estimated. The FA, WS, and FF with carbon and/or dry sorbent injection systems had 75{\%} to 82{\%} average removal efficiencies. On the other hand, the ESP with/without dry sorbent injection had lower removal efficiencies of up to 22{\%}. The type of dry sorbent injection in the FF system, dry or semi-dry, did not make more than 1{\%} difference to the removal efficiency. The injection of activated carbon and carbon-containing fly ash in the FF system made less than 3{\%} difference. Estimation errors of removal efficiency were especially high for the ESP. The national average of removal efficiency of APCDs in Japanese MSWI plants was estimated on the basis of incineration capacity. Owing to the replacement of old APCDs for dioxin control, the national average removal efficiency increased from 34.5{\%} in 1991 to 92.5{\%} in 2003. This resulted in an additional reduction of about 0.86. Mg emission in 2003. Further study using the methodology in this study to other important emission sources like coal-fired power plants will contribute to better emission inventories.",
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