Ultrafast electronic state conversion at room temperature utilizing hidden state in cuprate ladder system

R. Fukaya, Y. Okimoto, M. Kunitomo, K. Onda, T. Ishikawa, S. Koshihara, H. Hashimoto, S. Ishihara, A. Isayama, H. Yui, T. Sasagawa

Research output: Contribution to journalArticle

14 Citations (Scopus)

Abstract

Photo-control of material properties on femto-(10-15) and pico-(10-12) second timescales at room temperature has been a long-sought goal of materials science. Here we demonstrate a unique ultrafast conversion between the metallic and insulating state and the emergence of a hidden insulating state by tuning the carrier coherence in a wide temperature range in the two-leg ladder superconductor Sr14-xCaxCu24O41 through femtosecond time-resolved reflection spectroscopy. We also propose a theoretical scenario that can explain the experimental results. The calculations indicate that the holes injected by the ultrashort light reduce the coherence among the inherent hole pairs and result in suppression of conductivity, which is opposite to the conventional photocarrier-doping mechanism. By using trains of ultrashort laser pulses, we successively tune the carrier coherence to within 1 picosecond. Control of hole-pair coherence is shown to be a realistic strategy for tuning the electronic state on ultrafast timescales at room temperature.

Original languageEnglish
Article number8519
JournalNature communications
Volume6
DOIs
Publication statusPublished - Oct 20 2015

Fingerprint

Ladders
Electronic states
ladders
cuprates
Temperature
room temperature
electronics
Carrier State
Tuning
tuning
Spectrum Analysis
Leg
Lasers
Materials science
materials science
Ultrashort pulses
Superconducting materials
Light
Materials properties
Doping (additives)

All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Biochemistry, Genetics and Molecular Biology(all)
  • Physics and Astronomy(all)

Cite this

Ultrafast electronic state conversion at room temperature utilizing hidden state in cuprate ladder system. / Fukaya, R.; Okimoto, Y.; Kunitomo, M.; Onda, K.; Ishikawa, T.; Koshihara, S.; Hashimoto, H.; Ishihara, S.; Isayama, A.; Yui, H.; Sasagawa, T.

In: Nature communications, Vol. 6, 8519, 20.10.2015.

Research output: Contribution to journalArticle

Fukaya, R, Okimoto, Y, Kunitomo, M, Onda, K, Ishikawa, T, Koshihara, S, Hashimoto, H, Ishihara, S, Isayama, A, Yui, H & Sasagawa, T 2015, 'Ultrafast electronic state conversion at room temperature utilizing hidden state in cuprate ladder system', Nature communications, vol. 6, 8519. https://doi.org/10.1038/ncomms9519
Fukaya, R. ; Okimoto, Y. ; Kunitomo, M. ; Onda, K. ; Ishikawa, T. ; Koshihara, S. ; Hashimoto, H. ; Ishihara, S. ; Isayama, A. ; Yui, H. ; Sasagawa, T. / Ultrafast electronic state conversion at room temperature utilizing hidden state in cuprate ladder system. In: Nature communications. 2015 ; Vol. 6.
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AU - Koshihara, S.

AU - Hashimoto, H.

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