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研究成果 2001 2019

  • 1484 引用
  • 19 h指数
  • 50 記事
  • 37 会議での発言
2019

Alternative Ni-alloy cermet anode materials for SOFCs

Ishibashi, Y., Futamura, S., Tachikawa, Y., Matsuda, J., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2019, Solid Oxide Fuel Cells 16, SOFC 2019. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1889-1896 8 p. (ECS Transactions; 巻数 91, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Anodes
Energy conversion
Zirconia
Deterioration

Biogas Power Generation with SOFC to Demonstrate Energy Circulation Suitable for Mekong Delta, Vietnam

Shiratori, Y., Sakamoto, M., Nguyen, T. G. H., Yamakawa, T., Kitaoka, T., Orishima, H., Matsubara, H., Watanabe, Y., Nakatsuka, S., Doan, T. C. D. & Dang, C. M., 1 1 2019, : : Fuel Cells. 19, 4, p. 346-353 8 p.

研究成果: ジャーナルへの寄稿記事

Biogas
Solid oxide fuel cells (SOFC)
Power generation
Bagasse
Ponds
3 引用 (Scopus)

Development of paper-structured catalyst for application to direct internal reforming solid oxide fuel cell fueled by biogas

Nguyen, T. G. H., Sakamoto, M., Uchida, T., Doan, D. C. T., Dang, M. C., Tu, P. H., Sasaki, K. & Shiratori, Y., 4 23 2019, : : International Journal of Hydrogen Energy. 44, 21, p. 10484-10497 14 p.

研究成果: ジャーナルへの寄稿記事

Biogas
solid oxide fuel cells
Reforming reactions
Solid oxide fuel cells (SOFC)
catalysts

Fuel impurity poisoning of Ru/γ-Al2O3 catalyst packed in the reformer for biogas-fueled SOFC system

Setiawan, H., Yu, T. G., Nguyen, T. G. H., Sakamoto, M., Uchida, T. & Shiratori, Y., 1 1 2019, Solid Oxide Fuel Cells 16, SOFC 2019. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1651-1659 9 p. (ECS Transactions; 巻数 91, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Catalyst poisoning
Biogas
Solid oxide fuel cells (SOFC)
Impurities
Catalysts

Indirect internal reforming SOFC accommodating graded-catalytic domain fabricated by paper-structured catalyst

Aydın, Matsumoto, G., Kubota, A., Tran, D. L., Sakamoto, M. & Shiratori, Y., 1 1 2019, Solid Oxide Fuel Cells 16, SOFC 2019. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1631-1640 10 p. (ECS Transactions; 巻数 91, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Reforming reactions
Solid oxide fuel cells (SOFC)
Catalysts
Thermal stress
Flow fields
1 引用 (Scopus)
cell anodes
solid oxide fuel cells
Solid oxide fuel cells (SOFC)
Anodes
anodes
3 引用 (Scopus)

SOFC anodes impregnated with noble metal catalyst nanoparticles for high fuel utilization

Futamura, S., Muramoto, A., Tachikawa, Y., Matsuda, J., Lyth, S. M., Shiratori, Y., Taniguchi, S. & Sasaki, K., 3 29 2019, : : International Journal of Hydrogen Energy. 44, 16, p. 8502-8518 17 p.

研究成果: ジャーナルへの寄稿記事

公開
cell anodes
solid oxide fuel cells
Precious metals
Solid oxide fuel cells (SOFC)
noble metals

SOFC anodes impregnated with noble metal catalyst nanoparticles for high fuel utilization

Futamura, S., Muramoto, A., Tachikawa, Y., Matsuda, J., Lyth, S. M., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2019, Solid Oxide Fuel Cells 16, SOFC 2019. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1905-1913 9 p. (ECS Transactions; 巻数 91, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Precious metals
Solid oxide fuel cells (SOFC)
Anodes
Nanoparticles
Catalysts

Study on Ni-(Ce,Zr,M)O2-δ anode for direct internal reforming SOFC fueled by biogas

Takata, S., Sakamoto, M., Yamamoto, T., Tamazaki, F. & Shiratori, Y., 1 1 2019, Solid Oxide Fuel Cells 16, SOFC 2019. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1993-2000 8 p. (ECS Transactions; 巻数 91, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Biogas
Reforming reactions
Solid oxide fuel cells (SOFC)
Anodes
Methane
2018
5 引用 (Scopus)

Designing graded catalytic domain to homogenize temperature distribution while dry reforming of CH4

Aydın, Ö., Kubota, A., Tran, D. L., Sakamoto, M. & Shiratori, Y., 9 6 2018, : : International Journal of Hydrogen Energy. 43, 36, p. 17431-17443 13 p.

研究成果: ジャーナルへの寄稿記事

Reforming reactions
Flow fields
flow distribution
Temperature distribution
temperature distribution

Hydrothermal synthesis and characterisation of iron cerium oxide nanoparticles for hydrogen sulphide removal application

To, T. D., Nguyen, H. G. T., Doan, T. C. D., Shiratori, Y. & Dang, C. M., 1 1 2018, : : International Journal of Nanotechnology. 15, 11-12, p. 887-899 13 p.

研究成果: ジャーナルへの寄稿記事

cerium oxides
hydrogen sulfide
Hydrothermal synthesis
Cerium
iron oxides
8 引用 (Scopus)

Ni-loaded (Ce,Zr)O2–Δ-dispersed paper-structured catalyst for dry reforming of methane

Nguyen, T. G. H., Tran, D. L., Sakamoto, M., Uchida, T., Sasaki, K., To, T. D., Doan, D. C. T., Dang, M. C. & Shiratori, Y., 3 8 2018, : : International Journal of Hydrogen Energy. 43, 10, p. 4951-4960 10 p.

研究成果: ジャーナルへの寄稿記事

Coking
Reforming reactions
Methane
methane
catalysts
2017
3 引用 (Scopus)

Advanced direct internal reforming concepts for solid oxide fuel cells running with biogas

Tran, D. L., Kubota, A., Sakamoto, M., Tran, Q. T., Sasaki, K. & Shiratori, Y., 5 30 2017, ECS Transactions. Kawada, T. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 2467-2476 10 p. (ECS Transactions; 巻数 78, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Biogas
Reforming reactions
Solid oxide fuel cells (SOFC)
Anodes
Mechanical stability
8 引用 (Scopus)
Solid oxide fuel cells (SOFC)
Anodes
Catalysts
Nanoparticles
Impregnation
2 引用 (Scopus)

Alternative SOFC anode materials with ion- and electron-conducting backbones for higher fuel utilization

Futamura, S., Tachikawa, Y., Matsuda, J., Lyth, S. M., Shiratori, Y., Taniguchi, S. & Sasaki, K., 5 30 2017, ECS Transactions. 1 版 Electrochemical Society Inc., 巻 78. p. 1179-1187 9 p.

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Zirconia
Anodes
Electrons
Gadolinium
3 引用 (Scopus)

Biogas production from local biomass feedstock in the Mekong Delta and its utilization for a direct internal reforming solid oxide fuel cell

Shiratori, Y., Yamakawa, T., Sakamoto, M., Yoshida, H., Kitaoka, T., Tran, Q. T., Tin Doan, D. C. & Dang, M. C., 5 26 2017, : : Frontiers in Environmental Science. 5, MAY, 25.

研究成果: ジャーナルへの寄稿記事

fuel cell
biogas
oxide
biomass
methane
2 引用 (Scopus)

Degradation of SOFCs by various impurities: Impedance spectroscopy and microstructural analysis

Kikuchi, Y., Matsuda, J., Tachikawa, Y., Shiratori, Y., Taniguchi, S. & Sasaki, K., 5 30 2017, ECS Transactions. Kawada, T. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1253-1260 8 p. (ECS Transactions; 巻数 78, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Spectroscopy
Impurities
Degradation
Coal gas
3 引用 (Scopus)

Development of flexible catalyst material for internal dry reforming

Nguyen, T. G. H., To, T. D., Sakamoto, M., Doan, D. C. T., Dang, M. C., Tran, Q. T., Sasaki, K. & Shiratori, Y., 5 30 2017, ECS Transactions. 1 版 Electrochemical Society Inc., 巻 78. p. 2431-2439 9 p.

研究成果: 著書/レポートタイプへの貢献会議での発言

Reforming reactions
Catalysts
Solid solutions
Catalyst activity
Anodes
4 引用 (Scopus)
Hydrogen Sulfide
Biofuels
Steam reforming
Biogas
Hydrogen sulfide

Effect of exchange current density on current distribution at planar-type SOFC anodes

Takino, K., Tachikawa, Y., Shiratori, Y., Taniguchi, S. & Sasaki, K., 5 30 2017, ECS Transactions. Kawada, T. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1523-1531 9 p. (ECS Transactions; 巻数 78, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Anodes
Current density
Methane
Computer simulation
1 引用 (Scopus)

Fuel composition in pressurized SOFCs

Muramoto, A., Kikuchi, Y., Tachikawa, Y., Shiratori, Y., Taniguchi, S. & Sasaki, K., 5 30 2017, ECS Transactions. Kawada, T. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 2497-2504 8 p. (ECS Transactions; 巻数 78, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Gas fuels
Chemical analysis
Hydrogen
Carbon
9 引用 (Scopus)
Open circuit voltage
solid oxide fuel cells
Solid oxide fuel cells (SOFC)
open circuit voltage
diagrams
5 引用 (Scopus)

Modelling of CH4 multiple-reforming within the Ni-YSZ anode of a solid oxide fuel cell

Tran, D. L., Tran, Q. T., Sakamoto, M., Sasaki, K. & Shiratori, Y., 1 1 2017, : : Journal of Power Sources. 359, p. 507-519 13 p.

研究成果: ジャーナルへの寄稿記事

solid oxide fuel cells
Reforming reactions
yttria-stabilized zirconia
Solid oxide fuel cells (SOFC)
Anodes
5 引用 (Scopus)

Ru-based SOFC anodes: Preparation, performance, and durability

Sugimoto, J., Futamura, S., Kawabata, T., Lyth, S. M., Shiratori, Y., Taniguchi, S. & Sasaki, K., 3 9 2017, : : International Journal of Hydrogen Energy. 42, 10, p. 6950-6964 15 p.

研究成果: ジャーナルへの寄稿記事

cell anodes
solid oxide fuel cells
Solid oxide fuel cells (SOFC)
durability
hydrocarbon fuels
2016
3 引用 (Scopus)

Catalytic and electrochemical behaviour of solid oxide fuel cell operated with simulated-biogas mixtures

Dang-Long, T., Quang-Tuyen, T. & Shiratori, Y., 6 3 2016, Proceedings of the 3rd AUN/SEED-NET Regional Conference on Energy Engineering and the 7th International Conference on Thermofluids, RCEnE/THERMOFLUID 2015. American Institute of Physics Inc., 巻 1737. 060012

研究成果: 著書/レポートタイプへの貢献会議での発言

solid oxide fuel cells
anodes
greenhouse effect
fuel flow
heat engines
22 引用 (Scopus)
Biofuels
Biogas
solid oxide fuel cells
Reforming reactions
Solid oxide fuel cells (SOFC)
2015
8 引用 (Scopus)

Effectiveness of paper-structured catalyst for the operation of biodiesel-fueled solid oxide fuel cell

Quang-Tuyen, T., Kaida, T., Sakamoto, M., Sasaki, K. & Shiratori, Y., 6 1 2015, : : Journal of Power Sources. 283, p. 320-327 8 p., 20745.

研究成果: ジャーナルへの寄稿記事

Biofuels
solid oxide fuel cells
Biodiesel
Solid oxide fuel cells (SOFC)
catalysts
15 引用 (Scopus)

Hydrotalcite-dispersed paper-structured catalyst for the dry reforming of methane

Shiratori, Y., Sakamoto, M., Uchida, T., Le, H., Quang-Tuyen, T. & Sasaki, K., 9 14 2015, : : International Journal of Hydrogen Energy. 40, 34, p. 10807-10815 9 p.

研究成果: ジャーナルへの寄稿記事

Reforming reactions
Methane
Solid oxide fuel cells (SOFC)
methane
Biogas
7 引用 (Scopus)

In operando visualization of SOFC electrodes by thermography and visible light imaging

Tachikawa, Y., Sugimoto, J., Takada, M., Kawabata, T., Lyth, S. M., Shiratori, Y. & Sasaki, K., 1 1 2015, : : ECS Electrochemistry Letters. 4, 11, p. F61-F64

研究成果: ジャーナルへの寄稿記事

Solid oxide fuel cells (SOFC)
Visualization
Infrared imaging
Reforming reactions
Imaging techniques
5 引用 (Scopus)

Microstructural characterization of SrZrO3 formation and the influence to SOFC performance

Kanae, S., Toyofuku, Y., Kawabata, T., Inoue, Y., Daio, T., Matsuda, J., Chou, J. T., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2015, Solid Oxide Fuel Cells 14, SOFC 2015. Singhal, S. C. & Eguchi, K. (版). 1 版 Electrochemical Society Inc., p. 2463-2470 8 p. (ECS Transactions; 巻数 68, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Electrochemical properties
Durability
Cathodes
Sintering
5 引用 (Scopus)

Oxidation-induced degradation of SOFC Ni anodes at high fuel utilizations

Kawasaki, T., Sugimoto, J., Tachikawa, Y., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2015, Solid Oxide Fuel Cells 14, SOFC 2015. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 1345-1352 8 p. (ECS Transactions; 巻数 68, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Anodes
Degradation
Oxidation
Partial pressure

Performance of SOFC power unit assisted by paper-structured catalyst

Shiratori, Y., Sakamoto, M., Tran, Q. T., Uchiyama, Y. & Uchiyama, N., 1 1 2015, Solid Oxide Fuel Cells 14, SOFC 2015. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., p. 2783-2788 6 p. (ECS Transactions; 巻数 68, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Catalysts
Exhaust systems (engine)
Fibers
Hydrocarbons
1 引用 (Scopus)

Smart fuel cell demonstration project: A challenge to realize SOFC-powered campus

Sasaki, K., Taniguchi, S., Shiratori, Y., Hayashi, A., Oshima, T., Nishihara, M., Tachikawa, Y., Daio, T., Kawabata, T., Fujita, M. & Zaitsu, A., 1 1 2015, Solid Oxide Fuel Cells 14, SOFC 2015. Eguchi, K. & Singhal, S. C. (版). 1 版 Electrochemical Society Inc., 巻 68. p. 171-178 8 p.

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Fuel cells
Demonstrations
Hydrogen
Power generation

Theoretical study of inorganic carbonaceous species reaction with the surfaces of BaTiO3(001)

Rivera, D. S., Ishimoto, T., Quang-Tuyen, T., Shiratori, Y. & Koyama, M., 1 1 2015, Solid Oxide Fuel Cells 14, SOFC 2015. Singhal, S. C. & Eguchi, K. (版). 1 版 Electrochemical Society Inc., p. 3177-3185 9 p. (ECS Transactions; 巻数 68, 番号 1).

研究成果: 著書/レポートタイプへの貢献会議での発言

Carbon
Chemisorption
Solid oxide fuel cells (SOFC)
Density functional theory
Adsorption
1 引用 (Scopus)

Visualization of SOFC anode by dual imaging method using infrared and visible light cameras

Tachikawa, Y., Kawabata, T., Shiratori, Y. & Sasaki, K., 2015, Solid Oxide Fuel Cells 14, SOFC 2015. 1 版 Electrochemical Society Inc., 巻 68. p. 1115-1120 6 p.

研究成果: 著書/レポートタイプへの貢献会議での発言

Solid oxide fuel cells (SOFC)
Anodes
Temperature distribution
Visualization
Cameras
2014
3 引用 (Scopus)

Durability of a Segmented-in-Series Tubular SOFC with a (Ce, Sm)O 2 cathode interlayer: Influence of operating conditions

Kobayashi, Y., Tomida, K., Tsukuda, H., Shiratori, Y., Taniguchi, S. & Sasakid, K., 2 14 2014, : : Journal of the Electrochemical Society. 161, 3

研究成果: ジャーナルへの寄稿記事

solid oxide fuel cells
Solid oxide fuel cells (SOFC)
durability
interlayers
Durability

Hydrotalcite-dispersed paper-structured catalyst for dry reforming of methane

Kakihara, Y., Shiratori, Y., Sakamoto, M., Takada, M., Uchida, T., Le, H. & Sasaki, K., 1 1 2014, 20th World Hydrogen Energy Conference, WHEC 2014. Committee of WHEC2014, p. 1411-1415 5 p. (20th World Hydrogen Energy Conference, WHEC 2014; 巻数 2).

研究成果: 著書/レポートタイプへの貢献会議での発言

Reforming reactions
Solid oxide fuel cells (SOFC)
Methane
Catalysts
Electrochemical oxidation
36 引用 (Scopus)

SOFC durability against standby and shutdown cycling

Hanasaki, M., Uryu, C., Daio, T., Kawabata, T., Tachikawa, Y., Lyth, S. M., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2014, : : Journal of the Electrochemical Society. 161, 9

研究成果: ジャーナルへの寄稿記事

shutdowns
Solid oxide fuel cells (SOFC)
durability
Durability
Degradation
2013
10 引用 (Scopus)

Chemical degradation of SOFCs: External impurity poisoning and internal diffusion-related phenomena

Sasaki, K., Yoshizumi, T., Haga, K., Yoshitomi, H., Hosoi, T., Shiratori, Y. & Taniguchi, S., 1 1 2013, : : ECS Transactions. 57, 1, p. 315-323 9 p.

研究成果: ジャーナルへの寄稿記事

poisoning
Solid oxide fuel cells (SOFC)
Impurities
Degradation
degradation

Computational study of performance drop phenomena based on sulfur adsorption and desorption model in planar-type SOFCs

Tachikawa, Y., Hosoi, T., Nishimura, T., Shiratori, Y., Taniguchi, S. & Sasaki, K., 2013, : : ECS Transactions. 57, 1, p. 2841-2848 8 p.

研究成果: ジャーナルへの寄稿記事

Solid oxide fuel cells (SOFC)
Desorption
Sulfur
Adsorption
Numerical analysis

Development of direct internal reforming SOFC integrated with paper-structured catalyst fuelled by biofuels

Shiratori, Y., Sakamoto, M., Takahashi, Y., Wakita, Y., Takada, M., Ogura, T., Nakajima, H. & Sasaki, K., 1 1 2013, : : ECS Transactions. 57, 1, p. 2997-3004 8 p.

研究成果: ジャーナルへの寄稿記事

Biofuels
Reforming reactions
Solid oxide fuel cells (SOFC)
Biogas
Catalysts
2 引用 (Scopus)

Durability of SOFC against thermal and redox cycling

Hanasaki, M., Uryu, C., Taniguchi, S., Shiratori, Y. & Sasaki, K., 1 1 2013, : : ECS Transactions. 57, 1, p. 691-697 7 p.

研究成果: ジャーナルへの寄稿記事

Thermal cycling
Solid oxide fuel cells (SOFC)
durability
Durability
Degradation
1 引用 (Scopus)

Durability of SOFCs using inexpensive Ca-doped ZrO2 electrolytes

Toyofuku, Y., Hosoi, T., Kawabata, T., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2013, : : ECS Transactions. 57, 1, p. 807-813 7 p.

研究成果: ジャーナルへの寄稿記事

Solid oxide fuel cells (SOFC)
durability
electrolyte
Durability
Electrolytes
1 引用 (Scopus)

Effect of ceria addition in SOFC anodes on sulfur poisoning

Sugimoto, J., Kawabata, T., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2013, : : ECS Transactions. 57, 1, p. 1395-1400 6 p.

研究成果: ジャーナルへの寄稿記事

Cerium compounds
poisoning
Solid oxide fuel cells (SOFC)
Anodes
Sulfur
17 引用 (Scopus)

Feasibility of palm-biodiesel fuel for a direct internal reforming solid oxide fuel cell

Quang-Tuyen, T., Shiratori, Y. & Sasaki, K., 5 1 2013, : : International Journal of Energy Research. 37, 6, p. 609-616 8 p.

研究成果: ジャーナルへの寄稿記事

Reforming reactions
Biodiesel
Solid oxide fuel cells (SOFC)
Degradation
Acoustic impedance
2 引用 (Scopus)

In-plane distribution of carbon deposition on SOFCs

Nishimura, T., Kawabata, T., Tachikawa, Y., Shiratori, Y., Taniguchi, S. & Sasaki, K., 1 1 2013, : : ECS Transactions. 57, 1, p. 1593-1598 6 p.

研究成果: ジャーナルへの寄稿記事

Solid oxide fuel cells (SOFC)
Carbon
Kerosene
Reforming reactions
Anodes
15 引用 (Scopus)

In situ synthesis of Ni/MgO catalysts on inorganic paper-like matrix for methane steam reforming

Miura, S., Umemura, Y., Shiratori, Y. & Kitaoka, T., 8 1 2013, : : Chemical Engineering Journal. 229, p. 515-521 7 p.

研究成果: ジャーナルへの寄稿記事

Magnesium Oxide
Nickel oxide
Steam reforming
Magnesia
magnesium
water management
Water Management
Fuel Cell
Water management
Electrolyte
19 引用 (Scopus)

Paper-structured catalyst for the steam reforming of biodiesel fuel

Shiratori, Y., Quang-Tuyen, T., Umemura, Y., Kitaoka, T. & Sasaki, K., 8 30 2013, : : International Journal of Hydrogen Energy. 38, 26, p. 11278-11287 10 p.

研究成果: ジャーナルへの寄稿記事

Steam reforming
Biodiesel
steam
Sols
catalysts
17 引用 (Scopus)

Performance enhancement of biodiesel fueled SOFC using paper-structured catalyst

Shiratori, Y., Quang-Tuyen, T. & Sasaki, K., 8 6 2013, : : International Journal of Hydrogen Energy. 38, 23, p. 9856-9866 11 p.

研究成果: ジャーナルへの寄稿記事

solid oxide fuel cells
Biodiesel
Solid oxide fuel cells (SOFC)
catalysts
Catalysts