Characteristics of atmospheric aerosols containing heavy metals measured on Fukue Island, Japan

Takehiro Hidemori, Tomoki Nakayama, Yutaka Matsumi, Takashi Kinugawa, Akihiro Yabushita, Masafumi Ohashi, Takao Miyoshi, Satoshi Irei, Akinori Takami, Naoki Kaneyasu, Ayako Yoshino, Ryota Suzuki, Yayoi Yumoto, Shiro Hatakeyama

    研究成果: ジャーナルへの寄稿学術誌査読

    24 被引用数 (Scopus)

    抄録

    To investigate transport and chemical compositions of fine aerosols in the East Asian region, aerosol chemical components and their mixing states were measured at Fukue Island in the spring of 2010. Off-line chemical analyses using an ion chromatographic analyzer and an inductively coupled plasma-mass spectrometer for the aerosols sampled by a high volume sampler have also been conducted. The mixing state and temporal variation of number concentrations of the particles containing lead (Pb) and vanadium (V) were studied by using a laser ionization single-particle aerosol mass spectrometer (LISPA-MS). The temporal variation of number concentrations of particles containing Pb measured by the LISPA-MS is well consistent with those obtained by the chemical analysis of the aerosols sampled by the high volume sampler. The Pb-containing particles were classified into four types from the statistical analysis on the basis of the single-particle mass spectra with assists of laboratory experiments. It is estimated that 52% of observed particles containing Pb were originated from coal combustion. The concentration-weighted trajectory (CWT) analysis suggests that these particles are mainly transported from China continent. The V-containing particles were classified into three types. The 41% of V-containing particles were internally mixed with sea salt and the result of CWT analysis suggests that the potentially anthropogenic V-containing particles possibility emitted from ships are mixing with sea salt in the region that is highly loaded with sea salt in the Pacific Ocean.

    本文言語英語
    ページ(範囲)447-455
    ページ数9
    ジャーナルAtmospheric Environment
    97
    DOI
    出版ステータス出版済み - 11月 1 2014

    !!!All Science Journal Classification (ASJC) codes

    • 環境科学(全般)
    • 大気科学

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