Development of paper-structured catalyst for application to direct internal reforming solid oxide fuel cell fueled by biogas

T. G.H. Nguyen, M. Sakamoto, T. Uchida, D. C.T. Doan, M. C. Dang, P. H. Tu, Kazunari Sasaki, Yusuke Shiratori

研究成果: ジャーナルへの寄稿記事

2 引用 (Scopus)

抄録

A flexible paper-structured catalyst (PSC) that can be applied to the anode of a solid oxide fuel cell (SOFC) was examined for its potential to enable direct internal reforming (DIR) operation. The catalytic activity of three types of Ni-loaded PSCs: (a) without the dispersion of support oxide particles in the fiber network (PSC-A), (b) with the dispersion of (Mg,Al)O derived from hydrotalcite (PSC–B), and (c) with the dispersion of (Ce,Zr)O2-δ (PSC–C), for dry reforming of CH4 was evaluated at operating temperatures of 650–800 °C. Among the PSCs, PSC-C exhibited the highest CH4 conversion with the lowest degradation rate. The electrochemical performance of an electrolyte-supported cell (ESC) was evaluated under the flow of simulated biogas at 750 °C for cases without and with the PSCs on the anode. The application of the PSCs improved the cell performance. In particular, PSC-C had a remarkably positive effect on stabilizing DIRSOFC operation fueled by biogas.

元の言語英語
ページ(範囲)10484-10497
ページ数14
ジャーナルInternational Journal of Hydrogen Energy
44
発行部数21
DOI
出版物ステータス出版済み - 4 23 2019

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Biogas
solid oxide fuel cells
Reforming reactions
Solid oxide fuel cells (SOFC)
catalysts
Catalysts
Anodes
anodes
cells
operating temperature
Catalyst supports
catalytic activity
Catalyst activity
Electrolytes
electrolytes
degradation
Degradation
Oxides
fibers
oxides

All Science Journal Classification (ASJC) codes

  • Renewable Energy, Sustainability and the Environment
  • Fuel Technology
  • Condensed Matter Physics
  • Energy Engineering and Power Technology

これを引用

Development of paper-structured catalyst for application to direct internal reforming solid oxide fuel cell fueled by biogas. / Nguyen, T. G.H.; Sakamoto, M.; Uchida, T.; Doan, D. C.T.; Dang, M. C.; Tu, P. H.; Sasaki, Kazunari; Shiratori, Yusuke.

:: International Journal of Hydrogen Energy, 巻 44, 番号 21, 23.04.2019, p. 10484-10497.

研究成果: ジャーナルへの寄稿記事

Nguyen, T. G.H. ; Sakamoto, M. ; Uchida, T. ; Doan, D. C.T. ; Dang, M. C. ; Tu, P. H. ; Sasaki, Kazunari ; Shiratori, Yusuke. / Development of paper-structured catalyst for application to direct internal reforming solid oxide fuel cell fueled by biogas. :: International Journal of Hydrogen Energy. 2019 ; 巻 44, 番号 21. pp. 10484-10497.
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