Effects of morphology on the thermoelectric properties of Al-doped ZnO

Li Han, Ngo Van Nong, Wei Zhang, Le Thanh Hung, Tim Holgate, Kazunari Tashiro, Michitaka Ohtaki, Nini Pryds, Søren Linderoth

    研究成果: ジャーナルへの寄稿記事

    26 引用 (Scopus)

    抄録

    The nanoparticles of Al-doped ZnO were successfully grown into rod-like and platelet-like morphologies by soft chemical routes. These powders were consolidated using spark plasma sintering (SPS) technique. The samples consolidated from rods and platelets exhibited characteristic structures with preferential orientation while the sample consolidated from nanoparticles did not show any sign of preferential orientation. The measured ZT values along the preferred orientation directions were found to be 0.16 and 0.25 at 1223 K for the samples consolidated from rods and platelets, respectively. The sample consolidated from nanoparticles exhibited fine grains and highly distributed nanoprecipitates, resulting in a ZT value of 0.3 at 1223 K due to the lower thermal conductivity resulting from nanostructuring. Using the simple parabolic band model and Debye-Callaway thermal transport model, the anisotropic properties of the nanostructured samples were elucidated and the influence of the grain size and nanoprecipitates on the electron and phonon transport was analyzed and discussed in detail.

    元の言語英語
    ページ(範囲)12353-12361
    ページ数9
    ジャーナルRSC Advances
    4
    発行部数24
    DOI
    出版物ステータス出版済み - 3 11 2014

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    Platelets
    Nanoparticles
    Spark plasma sintering
    Powders
    Thermal conductivity
    Electrons

    All Science Journal Classification (ASJC) codes

    • Chemistry(all)
    • Chemical Engineering(all)

    これを引用

    Han, L., Van Nong, N., Zhang, W., Hung, L. T., Holgate, T., Tashiro, K., ... Linderoth, S. (2014). Effects of morphology on the thermoelectric properties of Al-doped ZnO. RSC Advances, 4(24), 12353-12361. https://doi.org/10.1039/c3ra47617k

    Effects of morphology on the thermoelectric properties of Al-doped ZnO. / Han, Li; Van Nong, Ngo; Zhang, Wei; Hung, Le Thanh; Holgate, Tim; Tashiro, Kazunari; Ohtaki, Michitaka; Pryds, Nini; Linderoth, Søren.

    :: RSC Advances, 巻 4, 番号 24, 11.03.2014, p. 12353-12361.

    研究成果: ジャーナルへの寄稿記事

    Han, L, Van Nong, N, Zhang, W, Hung, LT, Holgate, T, Tashiro, K, Ohtaki, M, Pryds, N & Linderoth, S 2014, 'Effects of morphology on the thermoelectric properties of Al-doped ZnO', RSC Advances, 巻. 4, 番号 24, pp. 12353-12361. https://doi.org/10.1039/c3ra47617k
    Han L, Van Nong N, Zhang W, Hung LT, Holgate T, Tashiro K その他. Effects of morphology on the thermoelectric properties of Al-doped ZnO. RSC Advances. 2014 3 11;4(24):12353-12361. https://doi.org/10.1039/c3ra47617k
    Han, Li ; Van Nong, Ngo ; Zhang, Wei ; Hung, Le Thanh ; Holgate, Tim ; Tashiro, Kazunari ; Ohtaki, Michitaka ; Pryds, Nini ; Linderoth, Søren. / Effects of morphology on the thermoelectric properties of Al-doped ZnO. :: RSC Advances. 2014 ; 巻 4, 番号 24. pp. 12353-12361.
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    abstract = "The nanoparticles of Al-doped ZnO were successfully grown into rod-like and platelet-like morphologies by soft chemical routes. These powders were consolidated using spark plasma sintering (SPS) technique. The samples consolidated from rods and platelets exhibited characteristic structures with preferential orientation while the sample consolidated from nanoparticles did not show any sign of preferential orientation. The measured ZT values along the preferred orientation directions were found to be 0.16 and 0.25 at 1223 K for the samples consolidated from rods and platelets, respectively. The sample consolidated from nanoparticles exhibited fine grains and highly distributed nanoprecipitates, resulting in a ZT value of 0.3 at 1223 K due to the lower thermal conductivity resulting from nanostructuring. Using the simple parabolic band model and Debye-Callaway thermal transport model, the anisotropic properties of the nanostructured samples were elucidated and the influence of the grain size and nanoprecipitates on the electron and phonon transport was analyzed and discussed in detail.",
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