We demonstrate that double spin coating, where a perovskite film is covered with another perovskite film, can increase substrate coverage from 81% to 97% along with an increase of film thickness from 151 ± 17 to 246 ± 18 nm. The increased substrate coverage by double coating improves the solar power conversion efficiency from 7.1 ± 0.6 to 10.3 ± 1.0%, an approximate 1.5-fold increase. Additionally, a double-coated film of higher substrate coverage exhibits amplified spontaneous emission (ASE) while a single-coated film of lower substrate coverage does not exhibit ASE. Double coating is an attractive method for increasing substrate coverage and improving solar power conversion and ASE.
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