Light Amplification in Molecules Exhibiting Thermally Activated Delayed Fluorescence

Hajime Nakanotani, Taro Furukawa, Takuya Hosokai, Takuji Hatakeyama, Chihaya Adachi

研究成果: Contribution to journalArticle

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To reduce the threshold current density and move closer toward the realization of future current-injection organic semiconductor lasers, the harvesting of triplet excitons is anticipated because 75% excitons are directly formed as triplet excited states under electrical excitation according to spin statics. However, the observation of light amplification in pure phosphorescent or thermally activated delayed fluorescence (TADF) materials has nor yet been reported even under optical excitation. Herein, light amplification was observed in the TADF emitter 9-([1,1′-biphenyl]-3-yl)-N,N,5,11-tetraphenyl-5,9-dihydro-5,9-diaza-13b-boranaphtho[3,2,1-de]anthracen-3-amine (DABNA-2). It is found that DABNA-2 possesses not only a large stimulated emission cross-section but also a favorable window for light amplification. These results indicate that TADF emitters can form a new category of laser dyes and are important candidates for the realization of an organic semiconductor laser.

元の言語英語
記事番号1700051
ジャーナルAdvanced Optical Materials
5
発行部数12
DOI
出版物ステータス出版済み - 6 16 2017

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Atomic and Molecular Physics, and Optics

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