Microwave EPR spectroscopy of cobalt-doped germanium cuprate

S. V. Demishev, A. V. Semeno, N. E. Sluchanko, N. A. Samarin, A. A. Pronin, Y. Inagaki, S. Okubo, H. Ohta, Y. Oshima, L. I. Leonyuk

研究成果: Contribution to journalArticle査読

12 被引用数 (Scopus)

抄録

Resonance magnetoabsorption spectra of CuGeO3 single crystals containing 2% Co impurity have been studied in the frequency range 60-360 GHz in magnetic fields of up to 16 T and in the temperature interval 2-60 K with the magnetic field B aligned parallel to the a crystallographic axis. In addition to the Cu2+ chain resonance, a new absorption line (unobserved previously in doped CuGeO3 and deriving apparently from the Co 2+ ions) was detected in EPR spectra. Quantitative analysis of the spectra suggests that the spin-Peierls transition occurs in about 10% Cu 2+ chains, while the spin-Peierls state in the remaining 90% chains is completely destroyed by cobalt doping. The results obtained reveal considerable deviations from the universally accepted scenario of CuGeO 3 doping and are discussed within alternative theoretical models, namely, the quantum critical behavior (based on the EPR theory for quasi-one-dimensional systems) and a three-dimensional antiferromagnet with the Néel temperature lowered by disorder.

本文言語英語
ページ(範囲)2238-2248
ページ数11
ジャーナルPhysics of the Solid State
46
12
DOI
出版ステータス出版済み - 2004
外部発表はい

All Science Journal Classification (ASJC) codes

  • 電子材料、光学材料、および磁性材料
  • 凝縮系物理学

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