In networks of spatially distributed fluorescent molecules, Förster resonance energy transfer (FRET) can simultaneously occur over multiple locations and times. Such "FRET networks"have great potential for information-processing and computing applications. To design these applications, the spatiotemporal behavior of FRET networks should be understood. However, studies on their spatiotemporal behavior are scarce. Here, we develop a spatiotemporal model for FRET networks and uncover its temporal characteristic behavior.We theoretically show that our model can generate a distinctive temporal behavior, i.e., the network-induced multicomponent exponential decay of the fluorescence intensity, even for FRET networks of fluorophores with an identical single exponential decay. This theoretical result is supported experimentally using quantum dots.
|ジャーナル||Journal of the Optical Society of America B: Optical Physics|
|出版ステータス||出版済み - 2 2021|
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